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Tytuł:
$[Ni(en)(H_2O)_4][SO_4] \cdot 2H_2O$ - an S = 1 Molecular Magnet with Easy-Plane Anisotropy
Autorzy:
Tarasenko, R.
Orendáčová, A.
Tibenská, K.
Potočňák, I.
Kajňaková, M.
Vlček, A.
Orendáč, M.
Feher, A.
Powiązania:
https://bibliotekanauki.pl/articles/1813818.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.30.Et
75.30.Gw
75.40.Cx
Opis:
Structural analysis of $[Ni(en)(H_2O)_4][SO_4] \cdot 2H_2O$ was performed and it suggests that the crystal field should play a dominant role in the magnetic properties of the system. This conjecture coincides well with the specific heat and susceptibility behaviour. The analysis confirmed that the compound can be treated as a spin 1 single molecule magnet with nonmagnetic ground state introduced by easy-plane single-ion anisotropy D/$k_B$≈11 K and neglecting in-plane anisotropy E/D <0.1.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 481-484
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
$Zn_{1-x}(Mn,Co)_xGeAs_2$ Ferromagnetic Semiconductor: Magnetic and Transport Properties
Autorzy:
Kilanski, L.
Gorska, M.
Domukhovski, V.
Dobrowolski, W.
Anderson, J.
Rotundu, C.
Varniavskii, S.
Marenkin, S.
Powiązania:
https://bibliotekanauki.pl/articles/1811937.pdf
Data publikacji:
2008-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
72.20.Fr
72.80.Ga
75.50.Pp
75.40.Cx
Opis:
We present the studies of magnetic and transport properties of the bulk $Zn_{1-x}(Mn, Co)_xGeAs_2$ mixed crystals with 0.052 ≤ x ≤0.182 grown using direct fusion method. Magnetic investigations showed that for samples with x ≥ 0.078 we observed a behavior typical of ferromagnets, with the Curie temperatures $T_C$ ≥ 300 K. The observed ferromagnetism was probably connected with the spinodal decomposition of the Mn ions in the alloy. The transport studies including resistivity and Hall effect (at B=1.4 T) were performed. The samples showed p-type conductivity with semiconducting or metallic character, depending on the alloy composition. The Hall carrier concentration, p ≥ $10^{18} cm^{-3}$, was composition dependent.
Źródło:
Acta Physica Polonica A; 2008, 114, 5; 1151-1157
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
A Coupled Spin-Electron Diamond Chain with Different Landé g-Factors of Localized Ising Spins and Mobile Electrons
Autorzy:
Torrico, J.
Pereira, M.
Strečka, J.
Lyra, M.
Powiązania:
https://bibliotekanauki.pl/articles/1032419.pdf
Data publikacji:
2017-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
05.50.+q
75.10.Pq
75.30.Kz
75.40.Cx
Opis:
A coupled spin-electron diamond chain with localized Ising spins placed on its nodal sites and mobile electrons delocalized over interstitial sites is explored in a magnetic field taking into account the difference between the Landé g-factors of the localized spins and mobile electrons. The ground-state phase diagram is constituted by two classical ferrimagnetic phases, the quantum unsaturated paramagnetic phase and the saturated paramagnetic phase. Both classical ferrimagnetic phases as well as the unsaturated paramagnetic phase are reflected in a low-temperature magnetization curve as intermediate magnetization plateaus. The unsaturated paramagnetic phase is quantum in its character as evidenced by the fermionic concurrence calculated for a pair of the mobile electrons hopping in between the interstitial sites. It is shown that the magnetic field can under certain conditions induce a quantum entanglement above the disentangled ground state.
Źródło:
Acta Physica Polonica A; 2017, 132, 1; 140-142
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
AC Magnetic Susceptibility Study of Fe and Co Based Nanoparticles
Autorzy:
Zeleňáková, A.
Kováč, J.
Zeleňák, V.
Powiązania:
https://bibliotekanauki.pl/articles/1368479.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.75.Fk
81.05.Rm
75.40.Cx
Opis:
We have investigated magnetic properties of three different samples composed of magnetic Fe or Co core and protective Au or Pt metallic shell, namely Fe@Au, Co@Au and Fe@Pt samples, with sizes of about 10 nm, 8 nm and 5 nm respectively. We have measured and analysed the experimental data of real and imaginary component of ac susceptibility through theoretical laws for non-interacting and interacting particles and we have estimated the strength of their magnetic interactions. Our analyses showed the increase of inter-particle interactions with decreasing particles size.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 222-223
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
An Enthalpy of Solution of Silicon in Iron Studied by $ \text{}^{57}$ Fe Mössbauer Spectroscopy
Autorzy:
Idczak, R.
Konieczny, R.
Chojcan, J.
Powiązania:
https://bibliotekanauki.pl/articles/1398353.pdf
Data publikacji:
2016-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
76.80.+y
75.50.Bb
82.60.Cx
82.60.Lf
Opis:
The room temperature Mössbauer spectra of $\text{}^{57}Fe$ were measured for $Fe_{1-x}Si_x$ solid solutions with x in the range 0.01 ≤ x ≤ 0.05. The obtained data were analysed in terms of the binding energy $E_{b}$ between two silicon atoms in the studied materials using the extended Hrynkiewicz-Królas idea. The extrapolated value of $E_{b}$ for x=0 was used to computation of an enthalpy of solution $H_{FeSi}$ of Si in α-Fe matrix. It was found that the $H_{FeSi}$ value is negative or Si atoms interact repulsively. The result was compared with corresponding values given in the literature which were derived from experimental calorimetric data as well as with the value resulting from the cellular atomic model of alloys by Miedema.
Źródło:
Acta Physica Polonica A; 2016, 129, 3; 367-370
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Anisotropy, Geometric Structure and Frustration Effects in Molecule-Based Nanomagnets
Autorzy:
Kamieniarz, G.
Kozłowski, P.
Antkowiak, M.
Sobczak, P.
Ślusarski, T.
Tomecka, D.
Barasiński, A.
Brzostowski, B.
Drzewiński, A.
Bieńko, A.
Mroziński, J.
Powiązania:
https://bibliotekanauki.pl/articles/1426672.pdf
Data publikacji:
2012-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.50.Xx
75.10.Jm
75.10.Pq
75.40.Cx
Opis:
In this paper we review our results of comprehensive study of molecular nanomagnets recently synthesized in the form of the chromium-based molecules and bimetallic copper-containing chains as well as we present some new findings. We focus on effects of anisotropy, geometry and frustration appearing in various thermodynamic properties of the nanoscale magnets which are described by Heisenberg-like spin models and simulated by accurate numerical methods. We show that bond-dependent exchange anisotropy is needed to model magnetic torque in the Cd-doped chromium ring. We argue that only in the limit of infinite rings (n → ∞) frustration can be considered as the opposite to bipartiteness in the odd numbered (3 ≤ n ≤ 9) s = 3/2 quantum spin rings. We analyse the influence of exchange interactions and anisotropy on magnetic susceptibility of bimetallic (S = 3/2, s = 1/2) chains composed of Cu ions linked to different 3d ions by fitting experimental data. We reach the remarkable consistency of the density functional theory estimates of the magnetic couplings in $Cr_8$ molecule and provide strong support to the spin models exploited in the literature.
Źródło:
Acta Physica Polonica A; 2012, 121, 5-6; 992-998
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Anomalous Magnetic Properties of URuGa
Autorzy:
Tran, V. H.
Troć, R.
Powiązania:
https://bibliotekanauki.pl/articles/1964580.pdf
Data publikacji:
1997-08
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
72.15.Qm
75.40.Cx
75.80.+q
Opis:
We present data of the magnetic susceptibility χ(T) and electrical resistivity ρ(T) for the hexagonal URuGa (space group P6̅2m). Below 7 K, χ increases rapidly and the data can be described by the expression χ(T) = χ(0)(1-a√T). ρ(T) in zero field follows the activated form: ρ(T)∼ exp(E$\text{}_{a}$/2k$\text{}_{B}$T ) with E$\text{}_{a}$ = 1.9 meV. In an applied magnetic field of 1 T, the resistivity varies as ρ(T)∼ bT. Between 18 and 250 K the resistivity is linear in -lnT and consistent with a Kondo-like effect.
Źródło:
Acta Physica Polonica A; 1997, 92, 2; 299-302
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Approximate Approach to Magnetic and Thermodynamic Properties of Mixed Spin (1/2-S) Chains with AB and $AB_2$ Topology
Autorzy:
Pełka, R.
Pinkowicz, D.
Powiązania:
https://bibliotekanauki.pl/articles/1534880.pdf
Data publikacji:
2010-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Pq
71.70.Gm
75.30.Cr
75.40.Cx
Opis:
Motivated by the rapid development in the synthesis of novel molecule-based magnets, we have investigated magnetic and thermodynamic properties of mixed spin (s-S) exchange coupled chains displaying a simple linear AB or a knotted $AB_2$ arrangement. Approximate approach for s = 1/2 and S ≥ 5/2, treating at an intermediate step spin S operator as a commuting variable and using the transfer matrix technique, is used. Susceptibility, magnetization and heat capacity of both spin systems are evaluated numerically from the corresponding free energy for S = 5/2. Uniform ferromagnetic and antiferromagnetic couplings are discussed. The procedure reproduces the right values of saturation magnetization and the entropy content of the systems, corroborating its correctness. χ T curves are shown to depend crucially on the $μ_{B}$ H/J ratio. For zero-field heat capacity a double-peak structure is revealed for the AB chain, whereas for the $AB_2$ chain only one broad anomaly is observed.
Źródło:
Acta Physica Polonica A; 2010, 118, 5; 959-961
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Breakdown of a Magnetization Plateau in Ferrimagnetic Mixed Spin-(1/2,S) Heisenberg Chains due to a Quantum Phase Transition towards the Luttinger Spin Liquid
Autorzy:
Strečka, J.
Powiązania:
https://bibliotekanauki.pl/articles/1032725.pdf
Data publikacji:
2017-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Pq
75.10.Kt
75.30.Kz
75.40.Cx
75.60.Ej
Opis:
Magnetization curves of the ferrimagnetic mixed spin-(1/2,S) Heisenberg chains are calculated with the help of density-matrix renormalization group method for several quantum spin numbers S=1, 3/2, 2 and 5/2. It is shown that the ferrimagnetic mixed spin-(1/2,S) Heisenberg chains exhibit irrespective of the spin value S exactly one intermediate magnetization plateau, which can be identified with the gapped Lieb-Mattis ferrimagnetic ground state. The magnetization plateau due to the Lieb-Mattis ferrimagnetism breaks down at a quantum phase transition towards the Luttinger spin liquid, which is characterized by a continuous change of the magnetization with the magnetic field until another quantum critical point is reached at the saturation field.
Źródło:
Acta Physica Polonica A; 2017, 131, 4; 624-626
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Chemical Potential as a Detector of Phase Transitions in Solids
Autorzy:
Matlak, M.
Gosławska, E.
Grabiec, B.
Eid, Kh.
Powiązania:
https://bibliotekanauki.pl/articles/2012963.pdf
Data publikacji:
2000-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
74.70.-b
75.30.Kz
75.40.Cx
Opis:
We show that the chemical potential exhibits small but distinct kinks at all critical temperatures as the evidence for phase transitions in the electronic system, structural phase transitions included. In the case of, at least, two kinds of interacting electrons average occupation numbers exhibit the same behavior.
Źródło:
Acta Physica Polonica A; 2000, 97, 3; 365-368
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Chemical Potential Derivative as Hallmark for Phase Transitions
Autorzy:
Pietruszka, M.
Matlak, M.
Powiązania:
https://bibliotekanauki.pl/articles/2011158.pdf
Data publikacji:
1999-12
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
64.60.-i
75.40.Cx
75.50.Ee
Opis:
We study antiferromagnetic properties of the two-band extended s-f model with fluctuating valence in the context of two mutually bound new effects of chemical potential critical behaviour, as well as of critical electron redistribution. In order to exemplify both phenomena we build phase diagrams of the system displaying the dependence of the critical Néel temperatures (T$\text{}_{N}$) of the system versus 4f (5f) level positions. The phase diagram consists of two different areas corresponding to antiferromagnetic and paramagnetic phases. We plot the magnetizations and the correlation functions of the system as functions of temperature. Next, we investigate the temperature dependence of the relative average occupation numbers Δn$\text{}^{f(d)}$ and the chemical potential Δμ for a given 4f (5f) level position E$\text{}_{f}$. Plotting this quantities along the E$\text{}_{f}$ cross-section lines we observe small (of the order of 10$\text{}^{-4}$-10$\text{}^{-3}$) but well localized kinks exactly at the Néel temperature T$\text{}_{N}$. Last but not least, we plot the first derivative of the chemical potential dμ/dT which, as it shows clearly visible jumps at T$\text{}_{N}$, may turn out to be very accurate and sensitive (auxiliary) tool to find critical temperatures of the considered system. Moreover, we plot the difference μ$\text{}_{AF}$-μ$\text{}_{PARA}$ where we subtract a chemical potential value of a reference paramagnetic sample from the actual value of the antiferromagnetic system. Also in this case we report the observation of discontinuous change in slope at T$\text{}_{N}$. Our observations can be extended to point out to a new practical possibility of how to find experimentally the critical temperatures of the antiferromagnetic systems exclusively from the chemical potential measurements. We expect that the same type of measurement, according to our recent and present results, would also apply to all types of critical phenomena in real solids.
Źródło:
Acta Physica Polonica A; 1999, 96, 6; 725-732
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Chemical Potential Evidence for Phase Transitions in Magnetic and Superconducting Compounds and Alloys
Autorzy:
Matlak, M.
Pietruszka, M.
Powiązania:
https://bibliotekanauki.pl/articles/2012914.pdf
Data publikacji:
2000-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
74.70.-b
75.30.Kz
75.40.Cx
Opis:
We announce that all phase transitions (induced by temperature or concentration) including structural ones and transitions between metastable or "exotic" states can be detected by the chemical potential critical behaviour, as well as, from the average occupation numbers of the electronic system (critical electron redistribution).
Źródło:
Acta Physica Polonica A; 2000, 97, 1; 253-256
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Complex Magnetic Behaviour of $Ho_3Cu_4X_4$ Compounds (X = Si and Sn)
Autorzy:
Gondek, Ł.
Szytuła, A.
Prokhnenko, O.
Powiązania:
https://bibliotekanauki.pl/articles/1813174.pdf
Data publikacji:
2008-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.25.+z
75.50.Ee
75.40.Cx
Opis:
Ternary $Ho_3Cu_4X_4$ compounds exhibit very complex magnetic phase diagrams. The rare earth ions occupy two non-equivalent crystal positions. Within both magnetic sublattices, magnetic moments exhibit different magnetic ordering temperatures. Moreover, in light of our results, it seems that both sublattices are weakly coupled between each other. This may be observed as independent changes of propagation vectors etc. The major difference of ordering temperatures between both compounds is likely related to substantial change of interatomic distances. Consequently, completely different crystalline electric field effects are observed.
Źródło:
Acta Physica Polonica A; 2008, 113, 4; 1179-1184
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Critical Behavior near the Ferromagnetic to Paramagnetic Phase Transition in Y₈Co₆₂B₃₀ Amorphous Alloy
Autorzy:
Śniadecki, Z.
Marcin, J.
Idzikowski, B.
Powiązania:
https://bibliotekanauki.pl/articles/1031033.pdf
Data publikacji:
2017-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.50.Kj
75.30.Sg
Opis:
The Y₈Co₆₂B₃₀ amorphous alloy is a collinear ferromagnet. The Arrott plot, the Kouvel-Fisher method, critical isotherm analysis and magnetic field dependence of maximum magnetic entropy changes were the main analytical tools used to determine the nature of the ferromagnetic/paramagnetic phase transition. Values of critical exponents (β, γ, and δ) were calculated and were convergent with those characteristic for mean-field model. It suggests that long range ferromagnetic interactions are playing main role in investigated alloy and the phase transition was confirmed to be of a second order according to the Banerjee criterion.
Źródło:
Acta Physica Polonica A; 2017, 131, 4; 967-969
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Critical Behaviour of the Mean-Field Ferromagnet $Cu_{1.02}[Cr_{1.77}Ti_{0.24}]Se_4$
Autorzy:
Krok-Kowalski, J.
Władarz, G.
Rduch, P.
Malicka, E.
Groń, T.
Guzik, A.
Powiązania:
https://bibliotekanauki.pl/articles/1409626.pdf
Data publikacji:
2012-12
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.50.Dd
64.60.Ht
Opis:
Magnetization, M, and susceptibility, χ, measurements showed both strong lowering of magnetic moment in comparison with $CuCr_2Se_4$ matrix and zero-field-cooling-field-cooling susceptibility splitting characteristic for the spin-glass behaviour. Isothermal magnetization curves, M(H), easy saturate and large values both of the Curie $T_{C}$=253 K and Curie-Weiss θ=283.5 K temperatures indicate the ferromagnetic order which coexists with the spin-glass state. The critical behaviour investigated around the paramagnetic-ferromagnetic phase transition revealed that the values of critical exponents are close to those predicted by the mean field model for long-range magnetic interactions.
Źródło:
Acta Physica Polonica A; 2012, 122, 6; 1102-1104
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
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