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Wyświetlanie 1-15 z 51
Tytuł:
Uniqueness of studies on electron densities in the extended momentum space
Autorzy:
Kontrym-Sznajd, G.
Powiązania:
https://bibliotekanauki.pl/articles/148018.pdf
Data publikacji:
2013
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
electron-positron momentum densities
Compton scattering
extended momentum space
positron annihilation
Opis:
This work draws attention to the fact that by measuring electronic structure via angular correlation of positron radiation (ACAR) and Compton scattering experiments one probes electron densities in the extended momentum space, directly related to the electron Bloch wave functions. Presenting some examples of electron densities in the extended and reduced momentum spaces, it is demonstrated what kind of information concerning the electronic structure can be obtained depending on the considered space. It is also shown how the knowledge of the symmetry selection rules allows to separate various Fermi surfaces and establish Fermi momenta.
Źródło:
Nukleonika; 2013, 58, 1; 203-206
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Understanding electron-positron momentum densities in solids : effect of the positron distribution
Autorzy:
Rubaszek, A.
Powiązania:
https://bibliotekanauki.pl/articles/147180.pdf
Data publikacji:
2015
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
electronic band structure
positron states
Opis:
The influence of the positron distribution on the electron-positron (e-p) momentum densities (MDs) is studied in terms of the l (l = s, p, d, f) character of the initial electronic state. The effect of the positron is discussed for momenta in the extended and reduced zone scheme on the example of Al (simple metal), Cu (metal with almost filled d shell), and Cr (transition metal). Present result indicates a weak sensitivity of the e-p MD inside the central Fermi surface to the positron charge density for the delocalized s and p electrons. In the case of d states, the effect of the positron on the relevant contribution to the e-p MD directly reflects the degree of localization of d electrons in the electron density of states.
Źródło:
Nukleonika; 2015, 60, No. 4, part 1; 759-763
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Track Effects in Positronium Formation
Autorzy:
Stepanov, S.
Byakov, V.
Duplâtre, G.
Stepanov, P.
Bokov, A.
Powiązania:
https://bibliotekanauki.pl/articles/1030026.pdf
Data publikacji:
2017-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
positron
positronium
annihilation
ion-electron recombination
solvation
mobility
external electric field
track effects
polar and nonpolar liquids
Opis:
We discuss some aspects important for interpretation of the Ps formation process in liquids and molecular media: (1) inhomogeneity of intratrack reactions and parameters of the e⁺ track, (2) final states of e⁺, its solvation in polar and nonpolar liquids, relation to e⁺ mobility, (3) quasi-neutrality of the e⁺ blob and its ambipolar outdiffusion, (4) appearance of the "in-blob" and "out-of-the-blob" positron fractions, and (5) electric field effect on Ps formation.
Źródło:
Acta Physica Polonica A; 2017, 132, 5; 1461-1465
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
The influence of hydrogen concentration on positron lifetime and electrical resistivity in vanadium-hydrogen systems
Autorzy:
Pietrzak, R.
Szatanik, R.
Powiązania:
https://bibliotekanauki.pl/articles/146289.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron lifetime
resistivity
V-H system
annihilation parameters
Opis:
Positron lifetime spectra and electrical resistivity of the vanadium-hydrogen systems with hydrogen concentration ranging from 0 to 0.29 at.H/at.V have been investigated. The range of hydrogen concentrations under investigation included the single alfa phase and a mixture of the alfa and beta phases of V-H system. The registered positron lifetime spectra were analysed by decomposition into two components. A distinct change in the annihilation parameters has been found after exceeding the boundary concentration of hydrogen in vanadium corresponding to the phase transition alfa (alfa+ beta). Correlation of changes in the parameters of the positron lifetime spectrum and in the electrical resistivity resulting from the changes in hydrogen concentration, has been revealed.
Źródło:
Nukleonika; 2010, 55, 1; 35-39
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
The influence of heat treatment on point defect concentration in Fe-Al and Fe-Al-Cr systems
Autorzy:
Kansy, J.
Hanc, A.
Giebel, D.
Powiązania:
https://bibliotekanauki.pl/articles/146336.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
Fe-Al
Fe-Al-Cr
point defects
Opis:
FeAl alloys of nominal Al content 28, 38 and 45 at.% and Fe28Al5Cr with minor alloying elements added to improve their application properties are studied by positron annihilation lifetime analysis. The lifetime spectra of samples FeXAl with X greater-than or equal to 38 (both quenched and cooled with furnace) are described by a single lifetime component related to the saturated positron trapping by quenched-in vacancies of concentration much higher than 100 ppm. A very strong dependence of retained vacancy concentration on the rate of cooling is shown for Fe28Al and Fe28Al5Cr alloys. After quenching, the concentration is of the order of 10.4 whereas in samples slowly cooled it is reduced to 10.5. The chromium addition to Fe28Al5Cr dismisses the vacancies concentration in comparison to the concentration in Fe28Al after the same heat treatment.
Źródło:
Nukleonika; 2010, 55, 1; 21-25
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Studies of unicellular microorganisms Saccharomyces cerevisiae by means of positron annihilation lifetime spectroscopy
Autorzy:
Kubicz, E.
Jasińska, B.
Zgardzińska, B.
Bednarski, T.
Białas, P.
Czerwiński, E.
Gajos, A.
Gorgol, M.
Kamińska, D.
Kapłon, Ł.
Kochanowski, A.
Korcyl, G.
Kowalski, P.
Kozik, T.
Krzemień, W.
Niedźwiecki, S.
Pałka, M.
Raczyński, L.
Rajfur, Z.
Rudy, Z.
Rundel, O.
Sharma, N. G.
Silarski, M.
Słomski, A.
Strzelecki, A.
Wieczorek, A.
Wiślicki, W.
Zieliński, M.
Moskal, P.
Powiązania:
https://bibliotekanauki.pl/articles/147902.pdf
Data publikacji:
2015
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
environmental scanning electron microscopy (ESEM)
free volume
inverted microscopy
positron annihilation
positronium
yeasts
Opis:
Results of positron annihilation lifetime spectroscopy (PALS) and microscopic studies on simple microorganisms, brewing yeasts, are presented. Lifetime of ortho-positronium (o-Ps) were found to change from 2.4 to 2.9 ns (longer-lived component) for lyophilized and aqueous yeasts, respectively. Also hygroscopicity of yeasts in time was examined, allowing to check how water – the main component of the cell – affects PALS parameters, thus lifetime of o-Ps were found to change from 1.2 to 1.4 ns (shorter-lived component) for the dried yeasts. The time sufficient to hydrate the cells was found below 10 hours. In the presence of liquid water, an indication of reorganization of yeast in the molecular scale was observed. Microscopic images of the lyophilized, dried, and wet yeasts with best possible resolution were obtained using inverted microscopy (IM) and environmental scanning electron microscopy (ESEM) methods. As a result, visible changes to the surface of the cell me mbrane were observed in ESEM images.
Źródło:
Nukleonika; 2015, 60, No. 4, part 1; 749-753
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Spektroskopia anihilacji pozytonow w Zjednoczonym Instytucie Badań Jądrowych w Dubnej
Positron Annihilation Spectroscopy at Joint Institute for Nuclear Research in Dubna
Autorzy:
Horodek, P.
Powiązania:
https://bibliotekanauki.pl/articles/214281.pdf
Data publikacji:
2016
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
spektroskopia anihilacji pozytonów
defekty struktury krystalicznej
wiązka powolnych pozytonów
przykłady zastosowań
positron annihilation spectroscopy
lattice defects
slow positron beam
examples of application
Opis:
W artykule przedstawiono spektroskopię anihilacji pozytonów, jako metodę dedykowaną do badań defektów struktury krystalicznej. Omówiono jej podstawy fizyczne i zaprezentowano technikę dopplerowskiego poszerzenia linii anihilacyjnej. Wskazano zakres stosowalności odnosząc się do najnowszych rozwiązań opartych na tzw. wiązkach powolnych pozytonów. Idea takiej wiązki, działającej w Laboratorium Problemów Jądrowych im. Dzhelepova w Zjednoczonym Instytucie Badań Jądrowych w Dubnej, została szerzej zaprezentowana. Przedstawiono zasadę działania oraz przykłady zastosowań z podstawami analizy otrzymywanych wyników.
Positron annihilation spectroscopy (PAS) as a method dedicated to study structural defects was presented. Physical basics of PAS and the Doppler broadening of annihilation line technique were discussed. Application range based on the newest technology, namely slow positron beams was presented. The idea of the beam, working at Dzhelepov Laboratory of Nuclear Problems at Joint Institute for Nuclear Research, along with the basic analysis of the results were described in details.
Źródło:
Postępy Techniki Jądrowej; 2016, 2; 18-23
0551-6846
Pojawia się w:
Postępy Techniki Jądrowej
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Principles of positron porosimetry
Autorzy:
Zaleski, R.
Powiązania:
https://bibliotekanauki.pl/articles/146520.pdf
Data publikacji:
2015
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
porous materials
positron annihilation lifetime spectroscopy (PALS)
positronium
extended Tao-Eldrup model
Opis:
The paper deals with positron porosimetry (PP), which is based on positron annihilation lifetime spectroscopy (PALS). The numerical analysis of positron lifetime spectra for PP is more demanding than in most of other applications of PALS. The resulting intensity distributions of ortho-positronium (o-Ps) lifetimes are interpreted in terms of the extended Tao-Eldrup (ETE) model, which provides the dependence between the o-Ps lifetime and pore size. Additionally, the relation between the intensity of an o-Ps component and the pore volume allows obtaining pore size distribution (PSD). The value of the empirical parameter Δ, which is dependent on material, can be estimated from the temperature dependence of an o-Ps lifetime. The most unique feature of PP among other techniques that allow determination of PSDs is its ability to perform measurements in almost any conditions. This makes this method suitable for various in situ studies. In this review article, both the capabilities and the limitations of PP are discussed. The methods to overcome some of the limitations are presented.
Źródło:
Nukleonika; 2015, 60, No. 4, part 1; 795-800
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron-annihilation and photoluminescence studies of nanostructured ZrO2
Autorzy:
Fidelus, J. D.
Karbowski, A.
Mariazzi, S.
Brusa, R. S.
Karwasz, G.
Powiązania:
https://bibliotekanauki.pl/articles/146313.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
zirconia nanopowders
photoluminescence
Opis:
In the present work, photoluminescence and Doppler broadening depth-resolved positron annihilation spectroscopy was performed on pure zirconia nanopowders. Zirconia nanopowders were grown by a hydrothermal microwave-driven process followed by annealing in oxygen atmosphere. Photoluminescence under 274 nm wavelength excitation from a 150 W high-pressure Xe exhibits similar spectra, in the region from 320 to 820 nm, although its intensity depends on the annealing. Positron annihilation Doppler-broadening spectra show low values of the normalized S-parameter, varying little with the depth, from 0.495 on the surface to 0.47-0.49 in bulk. Both high the annealing temperature and oxygen concentrations, lead to low bulk S-values. The ortho-positronium (o-Ps) fraction is about 10-11% for all samples on the surface, whereas it is reduced to 7-8% in the bulk for samples annealed at 700°C and 5-6% for samples annealed at 800°C. Both photoluminescence (PL) and positron studies show the presence of defects in all samples. The o-Ps signal suggests a high porosity of samples, particularly at a depth down to 10 nm.
Źródło:
Nukleonika; 2010, 55, 1; 85-89
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron study of the structure of nonadecane-tricosane mixed solid
Autorzy:
Zgardzińska, B.
Goworek, T.
Powiązania:
https://bibliotekanauki.pl/articles/146297.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
n-alkanes
binary mixture
Opis:
Positron annihilation lifetime and intensity were measured as a function of temperature for a binary mixture of two normal alkanes. The rotator phase is preceded by the range of about 7 K, in which one observes instability of spectrum parameters. In that range the mixed solid, being initially introduced into rotator phase, transforms to a rigid one in the time scale of several hours.
Źródło:
Nukleonika; 2010, 55, 1; 47-49
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron lifetime calculations for some elements on the base of the GGAPHNC approximation
Autorzy:
Boroński, E.
Powiązania:
https://bibliotekanauki.pl/articles/146330.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
electronic structure
Opis:
In studies of several interesting materials by positron annihilation technique the theoretical values of positron lifetimes in bulk and defected elements are useful. These lifetimes are often calculated within the GGA approximation. In this approximation the results of Arponen and Pajanne calculations for the positron in an electron gas are used. It is known, however, that when using the LDA approximation for the calculations of positron lifetime in real metals, Arponen and Pajanne values yield worse agreement with experimental data than the results obtained on the basis of PHNC formalism. Therefore, in this paper the appropriate PHNC formulas are incorporated into the GGA approximation and the calculations have been performed for some metals: bulk as well as containing monovacancies. The comparison of the lifetimes found in this way to the ones based on the previous method is promising for the applicability of the new algorithm.
Źródło:
Nukleonika; 2010, 55, 1; 9-12
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron annihilation study of structural relaxation and crystallization of glassified milk fat
Autorzy:
Rashevskaya, T.
Guly, I.
Pryadko, M.
Nishchenko, M.
Likhtorovich, S.
Powiązania:
https://bibliotekanauki.pl/articles/25394.pdf
Data publikacji:
2000
Wydawca:
Polska Akademia Nauk. Instytut Agrofizyki PAN
Tematy:
positron annihilation technique
milk fat
physical property
plasticity
consistency
crystallization
nutrition product
butter
amorphism
consistence zob.consistency
crystalline
elasticity
Źródło:
International Agrophysics; 2000, 14, 2
0236-8722
Pojawia się w:
International Agrophysics
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron annihilation study of iron oxide nanoparticles in mesoporous silica MCM-41 template
Autorzy:
Surowiec, Z.
Wiertel, M.
Zaleski, R.
Budzyński, M.
Goworek, J.
Powiązania:
https://bibliotekanauki.pl/articles/148449.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
Mössbauer effect
MCM-41 porous silica
superparamagnetic nanoparticles
Opis:
The subject of investigation were the samples obtained by impregnation of MCM-41 template with an aqueous solution prepared from Fe(NO3)3ź9H2O. As a result of such a procedure, iron oxides deposits on MCM-41 were formed. The Mössbauer studies revealed an occurrence of Fe3O4 nanocrystallites in the both ferri- and superparamagnetic states. Almost 80% small particles exist in a paramagnetic state. The positron annihilation lifetime spectroscopy (PALS) spectra were measured in air or in vacuum. The long-lived ortho-positronium (o-Ps) components and their intensities are time dependent due to air molecules interaction with iron oxide nanocrystallites and silica walls surfaces. The adsorption of air on the nanocrystallites surface causes a total screening of their surface and a raise of the o-Ps lifetime values. Observed anti-quenching effect is a result of competition of two phenomena: practically switching off a pick-off mechanism related to interaction of o-Ps with magnetite nanoparticles and considerably weaker usual quenching by paramagnetic oxygen molecules.
Źródło:
Nukleonika; 2010, 55, 1; 91-96
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron Annihilation Studies of the Free Volumes in Nylon12/PVA Films Treated by Supercritical Carbon Dioxide
Autorzy:
Li, Jingjing
Yin, Chongshan
Zhou, Yawei
Li, Gang
Yeh, Jen-taut
He, Chunqing
Powiązania:
https://bibliotekanauki.pl/articles/1033920.pdf
Data publikacji:
2017-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
Nylon12/PVA
ScCO₂
positron annihilation
free volume
relaxation
Opis:
Free volume variations of Nylon12/Polyvinyl alcohol (Nylon12/PVA) blends treated in supercritical carbon dioxide (ScCO₂) were investigated using positron annihilation lifetime spectroscopy. It is found that o-Ps lifetime τ₃ and the corresponding intensity I₃ in Nylon12/PVA decrease with increase of the PVA content. Being treated in ScCO₂ at 50°C and 20 MPa for 1 h, the free volume holes in Nylon12/PVA blends expand to different extents depending on the weight ratio of PVA. After releasing of CO₂, the free volume size decreases as a function of the elapsed time due to the molecular relaxation, and the relaxation time constant depends on the content of PVA in the blends.
Źródło:
Acta Physica Polonica A; 2017, 132, 5; 1552-1555
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron annihilation studies of mesoporous iron modified MCM-41 silica
Autorzy:
Wiertel, M.
Surowiec, Z.
Budzyński, M.
Gac, W.
Powiązania:
https://bibliotekanauki.pl/articles/147950.pdf
Data publikacji:
2013
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
iron
MCM-41 silica mesoporous materials
N2 sorption
positron annihilation
positron lifetime spectra
Opis:
MCM-41 silica materials modified by iron incorporation in the stage of its synthesis were investigated. The aim of the studies was determination of the nature of iron species and the influence of its content on the structural changes of materials and following the changes of their properties. For this purpose, the N2 sorption/desorption method and positron annihilation lifetime spectroscopy (PALS) were used. Disappearance of the longest-lived ortho-positronium (o-Ps) component (tau5) present in the PALS spectra of the initial MCM-41 material in the spectra of Fe-modified MCM-41 measured in vacuum is a result of a strong chemical o-Ps quenching and/or the Ps inhibition mechanism. Filling of pores by air or N2 at ambient pressure causes reappearance of the (tau5) component with lifetime shortened in comparison to that observed in vacuum for pure MCM-41 to the extent which can be explained by usual paramagnetic quenching in air. In contrary to the tendency observed for (tau5) lifetime which is practically independent of Fe content, the relevant intensity I5 monotonically decreases. This fact suggests that only inhibition of Ps formation occurs for the samples in air. Observed anti-quenching effect of air seems to be a result of competition of two processes : neutralization of surface active centres acting as inhibitors and considerably weaker paramagnetic quenching by O2 molecules.
Źródło:
Nukleonika; 2013, 58, 1; 245-250
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Wyświetlanie 1-15 z 51

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