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Wyświetlanie 1-15 z 87
Tytuł:
Magnetic Anisotropy of V$\text{}^{++}$ in CdS
Autorzy:
Herbich, M.
Mac, W.
Twardowski, A.
Demianiuk, M.
Powiązania:
https://bibliotekanauki.pl/articles/1950804.pdf
Data publikacji:
1996-10
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Dg
Opis:
The magnetization measurements at magnetic field up to 6 T obtained from newly grown hexagonal Cd$\text{}_{1-x}$V$\text{}_{x}$S (x ≈ 0.0004) are presented. The strong anisotropy of magnetization is observed at low temperatures (1.6 < T < 20 K). The data are well described by the crystal field model calculations taking into account static trigonal Jahn-Teller distortion and spin-orbit coupling.
Źródło:
Acta Physica Polonica A; 1996, 90, 4; 809-812
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Really First Principles Calculations for CoF₃
Autorzy:
Radwanski, R.
Nalecz, D.
Krupska, M.
Piwowarczyk, T.
Ropka, Z.
Powiązania:
https://bibliotekanauki.pl/articles/1385724.pdf
Data publikacji:
2015-02
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
76.30.Fc
75.10.Dg
Opis:
We have derived the low-energy electronic structure of CoF₃, originating from the strongly-correlated 3d⁶ system of the Co³⁺ ion, taking into account the crystal-field interactions, with a relatively weak trigonal distortion, and the relativistic spin-orbit interaction. We have calculated from really first-principles the relevant crystal-field interactions. With the discrete electronic structure for 3d electrons we have described the magnetic properties (the value of the magnetic moment and its direction). The moment direction is determined by the local off-octahedral trigonal distortion proving the single-ion origin of the magnetocrystalline anisotropy. We evaluated the orbital moment and the strength of spin interactions responsible for the formation of the magnetic state. Our studies indicate that calculations of the electronic structure of a 3d compound for the physically-adequate description of the magnetic properties has to be performed at the meV scale.
Źródło:
Acta Physica Polonica A; 2015, 127, 2; 391-393
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Crystal Field Theory of Magnetic Behaviour of Er$\text{}_{2}$(SO$\text{}_{4}$)$\text{}_{3}$·8H$\text{}_{2}$O
Autorzy:
Gupta, R.
Ghosh, U. S.
Basu, C.
Powiązania:
https://bibliotekanauki.pl/articles/1945413.pdf
Data publikacji:
1996-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.70.Ch
75.10.Dg
Opis:
Using the most rigorous approach of direct diagonalization of the Hamiltonian matrix constructed in the complete basis states (364 in number) of the Er$\text{}^{3+}$ ion the observed magnetic susceptibility and anisotropy data of erbium sulphate octahydrate were simulated and the set of crystal field parameters was evaluated. This procedure automatically includes the effect of intermediate coupling and the J-mixing under the crystal field. It was also demonstrated that such rigorous calculation using complete basis states is necessary in order to evaluate the correct set of parameters which may widely differ from the values obtained from approximate calculations previously performed using partial number of basis states of the ion concerned.
Źródło:
Acta Physica Polonica A; 1996, 89, 5-6; 649-655
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Stark and Zeeman Effects in Nd$\text{}_{2}$Fe$\text{}_{14}$B and Pr$\text{}_{2}$Fe$\text{}_{14}$B Intermetallics
Autorzy:
Radwański, R. J.
Franse, J. M.
Powiązania:
https://bibliotekanauki.pl/articles/1945558.pdf
Data publikacji:
1996-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.70.Ej
75.10.Dg
Opis:
The energy level scheme of the Nd$\text{}^{3+}$ and Pr$\text{}^{3+}$ ions in ferromagnetic Nd$\text{}_{2}$Fe$\text{}_{14}$B and Pr$\text{}_{2}$Fe$\text{}_{14}$B intermetallic compounds was evaluated on the basis of all known experiments. In calculations the effect of charge (Stark effect) and spin-dependent (Zeeman effect) interactions were taken into account by means of the crystal-field and molecular-field approximation, respectively. The derived energy level scheme is associated with the removal of the degeneracy of the lowest multiplet given by Hund's rules, i.e. $\text{}^{4}$I $\text{}_{9}\text{}_{/}\text{}_{2}$ (Nd$\text{}^{3+}$) and $\text{}^{3}$H$\text{}_{4}$ (Pr$\text{}^{3+}$). The revealed low-energy electronic structure (<25 meV = 200 cm$\text{}^{-1}$) is associated with many-electron states of the RE$\text{}^{3+}$ ions. Magnetic and electronic properties resulting from this fine structure are compared with all known experimental results. The localized crystal electric field levels exist also in Nd$\text{}_{2}$CuO$\text{}_{4}$, an ionic compound which by doping with Ce becomes high-T$\text{}_{c}$ superconductor, indicating the formation of crystal electric field states independently on the metallic or ionic state.
Źródło:
Acta Physica Polonica A; 1996, 90, 1; 223-232
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Atmospheric Pressure Plasma Jet for Mass Spectrometry
Autorzy:
Babij, M.
Gotszalk, T.
Kowalski, Z.
Nitsch, K.
Silberring, J.
Smoluch, M.
Powiązania:
https://bibliotekanauki.pl/articles/1198872.pdf
Data publikacji:
2014-06
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
52.50.Dg
82.80.Ms
Opis:
The atmospheric pressure plasma is much advantageous over low pressure plasmas in various aspects, e.g. vacuum-free operation, relative low cost, flexibility of a continuous process. Among various plasmas generated in atmospheric pressure discharges there are cold plasma jets that represent a technology of great application promise (industry, medicine, biology). To generate low-temperature plasmas at atmospheric pressure the dielectric barrier discharge can be used. It is suitable for the atomization of volatile species and can also be served as a ionization source for ambient mass and ion mobility spectrometry. As the discharge is generated in a restricted electrode structure, a plasma jet (plume) is usually formed outside the electrode region (that provides spatial separation of the plasma generation and surface processing regions). The paper presents a source based on a plasma jet established at the end of a capillary dielectric barrier discharge at atmospheric pressure and its application to mass spectrometry. The structure of the jet generator consists of piezoelectric transformer and two concentric and symmetric electrodes, between which the working gas flows at definite rate. Besides the source description early results of spectroscopic analysis are also given.
Źródło:
Acta Physica Polonica A; 2014, 125, 6; 1260-1262
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Theoretical Studies on the Local Structure and Spin Hamiltonian Parameters for Single Cu²⁺ Ion in BaF₂
Autorzy:
Lin, J.
Xiao, P.
Zhao, Y.
Zhang, B.
Yang, Y.
Powiązania:
https://bibliotekanauki.pl/articles/1398965.pdf
Data publikacji:
2016-06
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Dg
76.30.Fc
Opis:
The spin Hamiltonian parameters (g-factors and the hyperfine structure constants) and local structure are theoretically studied for single Cu²⁺ ion in BaF₂ from the high-order perturbation formulae of these parameters for 3d⁹ ions in tetragonally elongated octahedra. In the calculations, the ligand orbital and spin-orbit coupling of the impurity Cu²⁺ are taken into account, based on the cluster approach. Due to the Jahn-Teller effect and size mismatching substitution, the impurity Cu²⁺ is found to be located at a distance of about 0.2 Å from the nearest fluorine plane. The signs of the hyperfine structure constants $A_∥ $ and $ A_⊥ $ are suggested. The theoretical spin Hamiltonian parameters based on the above local structure are in good agreement with the observed values.
Źródło:
Acta Physica Polonica A; 2016, 129, 6; 1173-1177
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
The Systematic Variation of Optical Properties of Alkali Halides: an Ab Initio Study
Autorzy:
Gonçalves, G. C.
Lalic, M. V.
Malta, O. L.
Powiązania:
https://bibliotekanauki.pl/articles/2047877.pdf
Data publikacji:
2007-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.20.Dg
78.20.Ci
Opis:
In this paper we study a correlation between the optical properties, electronic structure and anion-cation electronegativity difference in three groups of alkali halides MX (M = Li, Na, K; X = F, Cl, Br, I). The electronic structure was calculated by first-principle, density-functional theory based full-potential linear augmented plane wave method. Then the complex dielectric function was computed, allowing determination of the optical absorption spectra in all compounds, up to incident radiation energy of 40 eV. The results were interpreted in terms of calculated band structures and correlated with the electronegativity difference in each compound, which was estimated on the basis of topological theory of Bader.
Źródło:
Acta Physica Polonica A; 2007, 112, 5; 1043-1048
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
The Effect of Water Accessible Paramagnetic Ions on Subcellular Structures Formed in Developing Wheat Photosynthetic Membranes as Observed by NMR and by Sorption Isotherm
Autorzy:
Harańczyk, H.
Leja, A.
Strzałka, K.
Powiązania:
https://bibliotekanauki.pl/articles/2044747.pdf
Data publikacji:
2006-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
82.56.Na
87.16.Dg
Opis:
The rehydration from the gaseous phase of the developing native or EDTA-washed from unbound and loosely bound paramagnetic ions wheat thylakoid membrane lyophilizate was investigated using hydration kinetics, sorption isotherm, and high power proton relaxometry. Hydration time courses are single exponential for all target humidities. The sorption isotherm is well fitted by the Dent model, with the mass of water saturating primary binding sites equal toΔ M/m$\text{}_{ }$0=0.024 and 0.017 for native and EDTA-washed membranes, respectively. Proton free induction decays distinguish: (i) a Gaussian component, S$\text{}_{0}$, coming from protons of solid matrix of lyophilizate; (ii) a Gaussian component, S$\text{}_{1}$, from water bound to the primary water binding sites in proximity of water accessible paramagnetic ions; (iii) an exponentially decaying contribution, $L$\text{}_{1}$$, from water tightly bound to lyophilizate surface; and (iv) exponentially decaying loosely bound water pool, L$\text{}_{2}$. Sorption isotherm fitted to NMR data shows a significant contribution of water "sealed" in membrane structures (Δ M$\text{}_{s}$/m$\text{}_{0}$=0.052 for native and 0.061 for EDTA-washed developing membranes, respectively).
Źródło:
Acta Physica Polonica A; 2006, 109, 3; 389-398
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Bound Water Structure on the Surfaces of Usnea antarctica as Observed by NMR and Sorption Isotherm
Autorzy:
Harańczyk, H.
Pietrzyk, A.
Leja, A.
Olech, M. A.
Powiązania:
https://bibliotekanauki.pl/articles/2044769.pdf
Data publikacji:
2006-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
82.56.Na
87.16.Dg
Opis:
Hydration courses and proton free induction decays are recorded at 30 MHz for Usnea antarctica thalli hydrated from gaseous phase. NMR data combined with gravimetry allow one to distinguish two fractions of tightly bound water, and loosely bound/free water pool. No water fraction "sealed" in thallus structures is present in U. antarctica.
Źródło:
Acta Physica Polonica A; 2006, 109, 3; 411-416
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Crystal-Field Interactions in $RPd_2Al_3$ Intermetallics (R = Pr, Nd, Sm, and U)
Autorzy:
Radwanski, R.
Nalecz, D.
Ropka, Z.
Powiązania:
https://bibliotekanauki.pl/articles/1374347.pdf
Data publikacji:
2014-10
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.70.Ej
75.10.Dg
Opis:
Magnetic and electronic properties of $NdPd_2Al_3$ have been nicely described with the $Nd^{3+}$ ions within the crystal-field theory revealing that all Nd atoms equally contribute to the temperature dependence of the paramagnetic susceptibility and of the heat capacity with the λ-peak. We consistently described paramagnetic and magnetically-ordered state. The fine electronic structure of the $Nd^{3+}$ ion nicely correlates with the electronic structure of the $U^{3+}$ ion in $UPd_2Al_3$ giving strong evidence for the trivalent uranium state in the isostructural heavy-fermion superconductor $UPd_2Al_3$.
Źródło:
Acta Physica Polonica A; 2014, 126, 4a; A-32-A-35
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Investigations on the EPR Parameters of $KMgF_3$:$Cr^{+}$
Autorzy:
Kuang, M.
Wu, S.
Hu, X.
Li, G.
Zu, H.
Powiązania:
https://bibliotekanauki.pl/articles/1365348.pdf
Data publikacji:
2014-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Dg
76.30.Fc
Opis:
The electron paramagnetic resonance parameters (i.e., g factor, hyperfine structure constant and superhyperfine parameters) of $KMgF_3$:$Cr^{+}$ are theoretically investigated from the perturbation formulae of these parameters for an octahedral $3 d^5$ cluster. As for the calculations of g factor and hyperfine structure constant, both the contributions from the crystal-field and charge transfer mechanisms are included based on the cluster approach. The metal to ligand charge transfer contribution to the g-shift Δg ( ≈ g-2.0023) is the same (negative) in sign and much larger in magnitude as compared to the crystal-field one. The conventional argument that the charge transfer contributions to zero-field splittings are negligible for $3 d^5$ ions in fluorides is no longer suitable for Δg analysis of $KMgF_3$:$Cr^{+}$ due to the dominant second-order charge transfer perturbation term. The charge transfer contribution to hyperfine structure constant exhibits the same sign and about 4% of the crystal-field one. The unpaired spin densities of the fluorine 2s, 2pσ and 2pπ orbitals are quantitatively acquired from the relationships with the relevant molecular orbital coefficients using the uniform model. The present treatments are superior to the previous calculations of directly fitting the experimental superhyperfine parameters.
Źródło:
Acta Physica Polonica A; 2014, 125, 5; 1224-1228
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
A Simple Localized-Itinerant Model for PrAl$\text{}_{3}$: Crystal Field and Exchange Effects
Autorzy:
Von Ranke, P. J.
Palermo, L.
Da Silva, X. A.
Powiązania:
https://bibliotekanauki.pl/articles/1891680.pdf
Data publikacji:
1991-10
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Dg
75.30.Cr
Opis:
We present a simple magnetic model for PrAl$\text{}_{3}$. The effects of crystal field are treated using a reduced set of levels and the corresponding wave functions are extracted from the actual crystal field levels of Pr$\text{}^{+3}$ in a hexagonal symmetry. The exchange between 4f- and conduction-electrons are dealt within a molecular field approximation. An analytical magnetic state equation is derived and the magnetic behaviour discussed. The parameters of the model are estimated from a fitting of the inverse susceptibility of PrAl$\text{}_{3}$ given in the literature.
Źródło:
Acta Physica Polonica A; 1991, 80, 4; 583-590
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Passive filter design for three-phase inverter interfacing in distributed generation
Autorzy:
Ahmed, K. H.
Finney, S. J.
Williams, B. W.
Powiązania:
https://bibliotekanauki.pl/articles/262578.pdf
Data publikacji:
2007
Wydawca:
Akademia Górniczo-Hutnicza im. Stanisława Staszica w Krakowie
Tematy:
DG
inverter
grid connected
filtering
damping
harmonics
Opis:
With the growing use of inverters in distributed generation, the problem of injected harmonics becomes critical. These harmonics require the connection of low pass filters between the inverter and the network. This paper presents a design method for the output LC filter in grid coupled applications in distributed generation systems. The design is according to the harmonics standards that determine the level of current harmonics injected into the grid network. Analytical expressions for the maximum inductor ripple current are derived. The filter capacitor design depends on the allowable level of switching components injected into the grid. Different passive filter damping techniques to suppress resonance affects are investigated and evaluated. Simulated results are included to verify the derived expressions.
Źródło:
Electrical Power Quality and Utilisation. Journal; 2007, 13, 2; 49-58
1896-4672
Pojawia się w:
Electrical Power Quality and Utilisation. Journal
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Impact of Vanadium(IV)-Oxy Acetylacetonate and Vanadium(III) Acetylacetonatel on the DPPC Liposome Membranes: EPR Studies
Autorzy:
Man, D.
Mrówka, I.
Wójcik, A.
Pytel, B.
Powiązania:
https://bibliotekanauki.pl/articles/1032414.pdf
Data publikacji:
2017-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
87.16.Dg
87.64.kh
87.80.Lg
Opis:
The effect of vanadium (IV)-oxy acetylacetonate (V4) and vanadium(III) acetylacetonate (V3) on the liposome membranes formed of synthetic lecithin (DPPC) was presented in this paper. Liposomes were formed during the sonication of DPPC lecithin in an aqueous medium. The concentration of the vanadium compounds changed in the range of 0% to 2.4% in molar ratio to the lecithin. The EPR technique made use of three spin probes penetrating the different areas of the membrane (as follows: TEMPO, 16-DOXYL stearic acid methyl ester, stearic acid 5-DOXYL methyl ester). TEMPO probe penetrates the interphase water-lipid (partition parameter F), the probe 16-DOXYL locates in the middle of the lipid bilayer (rotational correlation time τ), the probe 5-DOXYL gives a picture of membrane fluidity (the order parameter) just below the polar head groups. The results of our research showed the following conclusions. The change of membrane fluidity, as a function of admixture concentration, was dependent on the type of additives. TEMPO probe recorded an increase in liquidity interphase water-lipid for both admixtures: V3 and V4. 16-DOXYL probe indicated that the admixture V3 increases the fluidity in the center of the lipid bilayer. Admixture V4 significantly less impacted on the change of the membrane middle. The 5-DOXYL probe did not influence on the membrane surface portion, there were not observed significant changes under the impact of admixtures. V3 showed stronger impact on membrane fluidity.
Źródło:
Acta Physica Polonica A; 2017, 132, 1; 52-56
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Three localized f electrons in UPd₂Al₃ and in UGe₂ intermetallics
Autorzy:
Radwanski, R.
Nalecz, D.
Ropka, Z.
Powiązania:
https://bibliotekanauki.pl/articles/1062036.pdf
Data publikacji:
2016-08
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.70.Ej
75.10.Dg
75.30.Gw
Opis:
We have calculated the strength of the excitations between the crystal-field states which are in agreement with inelastic-neutron-scattering results. This agreement confirms the existence in the heavy-fermion superconductor UPd₂Al₃ the crystal-field electronic structure being the finger-print of the U^{3+} ions with three localized f electrons forming strongly-correlated atomic-like quantum system 5f³. The ionic integrity and the low-energy crystal-field electronic structure is preserved in this metallic system in the meV scale as has been postulated in the Quantum Atomistic Solid State theory (QUASST). We provide preliminary results with the U^{3+} ion in UGe₂ showing the ground-state eigenfunction which reproduces the ordered magnetic-moment value of 1.48 μ_{B}. This moment is composed from the dominant orbital contribution (2.6 μ_{B}) and the opposite spin moment (1.12 μ_{B}).
Źródło:
Acta Physica Polonica A; 2016, 130, 2; 545-550
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Wyświetlanie 1-15 z 87

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