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Tytuł:
Structure and Magnetic Properties of Three-Dimensional Gadolinium-Based Hybrid Framework
Autorzy:
Almáši, M.
Zeleňáková, A.
Císařová, I.
Bednarčík, J.
Zeleňák, V.
Powiązania:
https://bibliotekanauki.pl/articles/1371241.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.75.Fk
81.05.Rm
75.40.Cx
Opis:
In the present work we have focused on the preparation and magnetic study of coordination polymer formed by Gd(III) cations as nodes and formate (HCOO¯; FOR) anions as charge compensating linkers. The prepared complex with formula ${[Gd(μ_{3}-FOR)_{3}]}_{n}$ was characterized by single-crystal X-ray diffraction, and high-energy powder X-ray diffraction. The structural study showed that complex is formed by 3D polymeric network with the shortest Gd-Gd, distances of 3.998 Å. The magnetic properties of the complex were studied by magnetic susceptibility $χ_{M}(T)$ and magnetization M(H) measurements. The results show on the weak antiferromagnetic coupling at low temperatures represented by the Weiss constant θ=-0.468 K. The value of effective magnetic moment $μ_{eff}=7.57μ_{B}$, which was estimated from the experimental data is close to the theoretical value for systems with S=7/2. Correlation between crystal structure of complexes and magnetic properties is presented.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 308-309
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Modeling of the Experimental Molecular-Based Ring-Shaped Nanomagnets
Autorzy:
Antkowiak, M.
Kozłowski, P.
Musiał, G.
Florek, W.
Kamieniarz, G.
Esposito, F.
Powiązania:
https://bibliotekanauki.pl/articles/1534905.pdf
Data publikacji:
2010-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.40.Mg
Opis:
Quantum transfer matrix technique and numerically exact diagonalization method are applied to the Heisenberg spin systems to model ring-shaped molecules. Two cases are investigated: (i) a dozen of S = 1 spins with additional biquadratic exchange and (ii) a dimetallic molecule $Cr_7Cd$, where it is assumed that exchange anisotropy is determined in a local coordination system. In the latter case the calculated susceptibility is compared with experimental results.
Źródło:
Acta Physica Polonica A; 2010, 118, 5; 965-966
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Zero Temperature Magnetic Frustration in Nona-Membered s=3/2 Spin Rings with Bond Defect
Autorzy:
Antkowiak, M.
Kozłowski, P.
Kamieniarz, G.
Powiązania:
https://bibliotekanauki.pl/articles/1427128.pdf
Data publikacji:
2012-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.10.Jm
Opis:
Zero-temperature limits of the local and global thermodynamic quantities in the nine-membered antiferromagnetic s=3/2 spin ring are investigated by means of numerical exact diagonalization. An anisotropic Heisenberg model with tunable bond defect reflecting continuously varying topology (from closed to open ring) is exploited. The frustrated and non-frustrated phases are identified in the ground-state phase diagram determined by a bond-defect strength and magnetic field. Near the phase boundaries significance of the thermal fluctuations affecting the estimates of the local magnetic quantities found earlier at T=1 K is revealed. For the global quantities the effects of thermal fluctuations are found much weaker. A sequence of the local magnetic moments is analysed and their experimental verification at the edges of the non-frustrated and within the entire frustrated phase is suggested at sufficiently low temperature.
Źródło:
Acta Physica Polonica A; 2012, 121, 5-6; 1102-1104
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
New S=1/2 Alternating Chain Compound - High Pressure Form of (VO)$\text{}_{2}$P$\text{}_{2}$O$\text{}_{7^{-}}$
Autorzy:
Azuma, M.
Saito, T.
Hiroi, Z.
Takano, M.
Narumi, Y.
Kindo, K.
Powiązania:
https://bibliotekanauki.pl/articles/2012882.pdf
Data publikacji:
2000-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Jm
75.40.Cx
75.50.Ee
Opis:
The high-pressure phase of (VO)$\text{}_{2}$P$\text{}_{2}$O$\text{}_{7}$ comprises a unique kind of spin-1/2 Heisenberg alternating antiferromagnetic chain, in contrast with the ambient pressure phase containing two crystallographically different chains. Magnetic susceptibility and high-field magnetization data showed the presence of a single spin gap of 23 (magnetization) ~27 (susceptibility) K, not double as observed for the ambient pressure phase. This result shows that the two kinds of chains of the ambient pressure phase have single, different spin gaps.
Źródło:
Acta Physica Polonica A; 2000, 97, 1; 205-208
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Low Temperature Anomalies in the Specific Heat and Magnetic Susceptibility of $Na_{0.7}CoO_2$ Samples
Autorzy:
Baran, A.
Zorkovská, A.
Feher, A.
Šebek, J.
Šantavá, E.
Hejtmánek, J.
Veverka, M.
Bradarić, I.
Ružička, M.
Powiązania:
https://bibliotekanauki.pl/articles/1813849.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
72.80.Ga
Opis:
We present a comparative study of $Na_{0.7}CoO_2$ samples obtained from three different sources and prepared by different methods. The specific heat and magnetic susceptibility measurements in the temperature range 2-300 K show substantial influence on the observed anomalies, which underlines that the system is extremely sensitive to preparation protocols.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 495-498
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Thermodynamic and Magnetotransport Properties of High Quality $Na_{0.77}CoO_{2}$ Single Crystals
Autorzy:
Baran, A.
Zorkovská, A.
Kajňaková, M.
Lin, C.
Feher, A.
Powiązania:
https://bibliotekanauki.pl/articles/1371577.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.20.Hr
75.40.Cx
75.47.-m
Opis:
Heat capacity and electrical resistivity of high-quality $Na_{0.77}CoO_{2}$ single crystals was systematically studied as a function of temperature and magnetic field. Anomalies at 20 K have been observed both in the heat capacity and the electrical resistivity. The broad bump in the heat capacity indicates a smeared magnetic phase transition. Magnetic fields up to 9 T, oriented perpendicularly to the ab plane, reduce the temperature of this anomaly in accordance with the assumption of A-type antiferromagnetic ordering. The low temperature upturn observed in resistivity below 20 K for slow cooling is also suppressed by the magnetic field. This anomaly is probably the consequence of the interplay of several different mechanisms, including the Kondo effect, electron-electron interactions, and electron-phonon scattering.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 360-361
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic Properties of Spin-Ladders (A$\text{}_{2}$Cu$\text{}_{2}$O$\text{}_{3}$)$\text{}_{m}$ (CuO$\text{}_{2}$)$\text{}_{n}$
Autorzy:
Baran, M.
Szymczak, H.
Szymczak, R.
Dyeyev, S.
Leonyuk, L.
Babonas, G.-J.
Powiązania:
https://bibliotekanauki.pl/articles/2013220.pdf
Data publikacji:
2000-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.30.Gw
75.45.+j
75.90.+w
Opis:
Magnetization M(T) and M(H) data of single crystals of the S=1/2 quasi-one-dimensional system (A$\text{}_{2}$Cu$\text{}_{2}$O$\text{}_{3}$)$\text{}_{m}$(CuO$\text{}_{2}$)$\text{}_{n}$ with various A-site constituents are compared. The studied orthorhombic, incommensurate crystals are characterized by m/n=5/7,7/10, and 9/13. The role of rare-earth ions located in A-sites is discussed.
Źródło:
Acta Physica Polonica A; 2000, 97, 3; 571-574
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetism and Specific Heat of TmRhX (X = Ga, Ge) Compounds
Autorzy:
Baran, S.
Przewoźnik, J.
Szytuła, A.
Powiązania:
https://bibliotekanauki.pl/articles/1399029.pdf
Data publikacji:
2013-12
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.30.-m
75.30.kz
75.40.Cx
75.47.Np
Opis:
Magnetic and specific heat data of the TmRhX (X = Ga, Ge) compounds are reported. These compounds crystallize in an orthorhombic crystal structure of the TiNiSi-type (space group Pnma). Magnetic data indicate that the compounds are antiferromagnets with the Néel temperature $T_{N}$ equal to 3.9 K for TmRhGa and 6.0 K for TmRhGe. Magnetic susceptibility of TmRhGe has an additional peak at $T_{t}$ = 10.6 K. In TmRhGe temperature dependence of χ"(T), the positions of both the peaks at $T_{N}$ and $T_{t}$ change with frequency indicating a relaxation process. These data suggest that with the decreasing temperature, first a cluster glass state and next the long-range aniferromagnetic order exists.
Źródło:
Acta Physica Polonica A; 2013, 124, 6; 998-1001
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic and Neutron Diffraction Studies of the Polycrystalline and Nanoparticle $TbMnO_3$
Autorzy:
Bażela, W.
Dul, M.
Dyakonov, V.
Gondek, Ł.
Hoser, A.
Hoffmann, J.
Penc, B.
Szytuła, A.
Kravchenko, Z.
Nosalev, I.
Zarzycki, A.
Powiązania:
https://bibliotekanauki.pl/articles/1419577.pdf
Data publikacji:
2012-08
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.47.Lx
75.25.-j
75.50.Ee
Opis:
This paper reports on investigations of magnetic properties, crystal and magnetic structures on $TbMnO_3$ prepared in various ways, namely, as conventional polycrystalline sample and two nano particle specimens (synthesized with a sol-gel method at temperatures of 800 and 850°C). The X-ray and neutron diffraction data confirm the orthorhombic crystal structure (space group Pbnm, No. 62) without noticeable differences of the lattice parameters for poly- and nanocompounds. For the polycrystalline sample, a subsequent ordering of the Mn and Tb sublattices with decreasing temperature was observed. Namely, the Mn sublattice exhibits a modulated magnetic structure with the propagation vector k = (0, $k_{x},$ 0) in between 41-5 K. Below T = 21 K, a change from a collinear ($A_{y}$ mode) into non-collinear ($A_{y}G_{z}$ mode) structure was evidenced. Further decreasing of temperature below 10 K results in magnetic ordering of the Tb sublattice (modulated $G_{x}A_{y}F_{z}$ mode). For nanoparticle compounds, magnetic ordering in the Mn and Tb sublattices is described by propagation vector k = (0, $k_{y},$ 0), with $k_{y}$ components higher than observed for polycrystalline sample. The magnetic ordering in the Mn sublattice is described by a collinear $A_{y}$ mode down to 1.6 K where the Tb moment becomes ordered ($G_{x}A_{y}$ mode). The observed broadening of the Bragg peaks connected to the Tb sublattice suggests the cluster-like character of its magnetic structure.
Źródło:
Acta Physica Polonica A; 2012, 122, 2; 384-390
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Susceptibility Behaviour of CuGeO$\text{}_{3}$: Comparison between Experiment and the Quantum Transfer Matrix Approach
Autorzy:
Bieliński, M.
Renard, J.-P.
Powiązania:
https://bibliotekanauki.pl/articles/2013702.pdf
Data publikacji:
2000-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.10.Jm
75.40.Cx
75.40.Mg
Opis:
Thermodynamical properties of one-dimensional S=1/2 Heisenberg model with dimerized nearest- and uniform next-nearest-neighbour interactions are studied by the numerically exact quantum transfer matrix method and the results are applied to CuGeO$\text{}_{3}$. Suzuki-Trotter formula is used to obtain a classical system with spin σ=3/2 and effective interactions between nearest-neigbours only. Magnetic susceptibility curve is calculated and compared with new experimental results performed in a wide temperature range, revealing the presence of frustration in the model proposed for CuGeO$\text{}_{3}$.
Źródło:
Acta Physica Polonica A; 2000, 97, 5; 851-854
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic properties of the RbNd(WO₄)₂ single crystal
Autorzy:
Borowiec, M.
Zubov, E.
Zajarniuk, T.
Barański, M.
Powiązania:
https://bibliotekanauki.pl/articles/1075349.pdf
Data publikacji:
2016-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.50.Ee
75.10.-b
Opis:
The magnetic investigations as a function of the temperature and magnetic field for the rubidium neodymium double tungstate RbNd(WO₄)₂ single crystal have been performed. The magnetization was measured in the temperature range from 4.2 to 100 K and for the magnetic field up to 1.5 T. The crystal field and exchange parameters were found.
Źródło:
Acta Physica Polonica A; 2016, 129, 3; 359-361
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Direct Simulations of the Quantum Model for CsNiF$\text{}_{3}$
Autorzy:
Caramico D'Auria, A.
Esposito, F.
Esposito, U.
Kamieniarz, G.
Dekeyser, R.
Powiązania:
https://bibliotekanauki.pl/articles/1930597.pdf
Data publikacji:
1994-02
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
64.60.Cn
75.10.Dg
75.10.Jm
75.40.Cx
75.40.Mg
Opis:
We address the problem of reliability of a finite-chain technique for CsNiF$\text{}_{3}$. We investigate the effect of the boundary conditions, completely neglected so far, and apply a new extrapolation procedure appropriate for quantities showing non-monotonic behaviour. From a detailed analysis of the specific heat existing theoretical estimates for the model parameters are discriminated and a strong evidence for the reliability of the direct finite-chain technique predictions is presented.
Źródło:
Acta Physica Polonica A; 1994, 85, 2; 409-412
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Transition from Mixed-Valence to Trivalent Cerium State in Ce(Ni,Cu)Al Series
Autorzy:
Čermák, P.
Javorský, P.
Šantavá, E.
Powiązania:
https://bibliotekanauki.pl/articles/1534620.pdf
Data publikacji:
2010-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
75.30.Mb
Opis:
In this work we present the study of the part of Ce(Ni,Cu)Al series from the pure CeNiAl to 30% of copper concentration, which illustrates the transition from mixed-valence state of CeNiAl to the trivalent state in CeCuAl. The work is based on X-ray diffraction, magnetization and specific heat measurement. The results indicate smooth transition between the mixed-valence and trivalent cerium state. The specific-heat data reveal increase of the Sommerfeld γ coefficient with copper concentration.
Źródło:
Acta Physica Polonica A; 2010, 118, 5; 926-928
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Experimental Studies of S=1 Heisenberg Planar Antiferromagnetic Chain Ni(C$\text{}_{11}$H$\text{}_{10}$N$\text{}_{2}$O)$\text{}_{2}$Ni(CN)$\text{}_{4}$
Autorzy:
Čizmár, E.
Černák, J.
Orendáč, M.
Herrmannsdörfer, T.
Feher, A.
Powiązania:
https://bibliotekanauki.pl/articles/2013230.pdf
Data publikacji:
2000-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
71.20.Be
75.50.Ee
Opis:
In this paper we discuss the results of experimental studies of specific heat and magnetic susceptibility of chain compound Ni(C$\text{}_{11}$H$\text{}_{10}$N$\text{}_{2}$O)$\text{}_{2}$Ni(CN)$\text{}_{4}$. We have observed a Schottky type anomaly at T=2.2 K in a temperature dependence of specific heat and the compound was identified as a S=1 Heisenberg antiferromagnetic chain with the subcritical exchange coupling D/k$\text{}_{B}$=5 K, D/|J|=5.2 and the strong in-plane anisotropy E/k$\text{}_{B}$=2.8 K. It has been found that the in-plane anisotropy affects the region of validity of a diluted exciton model [1] and a strong coupling model [2] for S=1 Heisenberg chains with the strong planar anisotropy. The analysis suggests that the in-plane anisotropy should be considered in any attempt to find a compound potentially located in the boundary of Haldane and "large-D" phases.
Źródło:
Acta Physica Polonica A; 2000, 97, 3; 579-582
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Lattice Heat Capacity in RTAl (R = Y, Lu;T = Ni, Cu, Pd) Compounds
Autorzy:
Daniel, P.
Javorský, P.
Prchal, J.
Daniš, S.
Šantavá, E.
Powiązania:
https://bibliotekanauki.pl/articles/1813674.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
75.40.Cx
Opis:
We present analysis of the specific heat of the RTAl (R = Y, Lu;T = Cu, Ni, Pd) compounds. We focus on the lattice contribution and analyze the dependence of all the characteristic parameters in the Debye and Einstein models on the atomic masses and interatomic distances.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 331-334
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Wyświetlanie 1-15 z 100

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