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    Wyświetlanie 1-5 z 5
    Tytuł:
    Optical in situ Study of Reduction/Oxidation Processes in Cr,Mg:YAG Epitaxial Film
    Autorzy:
    Buryy, O.
    Ubizskii, S.
    Syvorotka, I.
    Becker, K.
    Powiązania:
    https://bibliotekanauki.pl/articles/1550540.pdf
    Data publikacji:
    2010-01
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    61.72.Cc
    66.30.Dn
    66.30.hd
    78.30.Hv
    78.40.Ha
    Opis:
    The changes of the optical absorption spectra of Cr,Mg:YAG epitaxial film caused by high-temperature redox treatment are investigated by means of in situ spectroscopy. The spectra were registered in the visible and near-IR spectral regions at temperatures up to 1100 K. The kinetics of optical absorption changing were obtained in the temperature range from 936 K to 1091 K and were described by mathematical model connecting the chromium recharging process with oxygen vacancies diffusion. The parameters of the model were determined from the approximations of the experimental kinetics.
    Źródło:
    Acta Physica Polonica A; 2010, 117, 1; 184-188
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Domain h Type Collective Dimerization of Graphite and Possible $sp^2$ rightarrow $sp^3$ Transition Induced by Inter h Layer Charge Transfer Excitations in the Visible Region
    Autorzy:
    Radosinski, L.
    Ostasiewicz, K.
    Luty, T.
    Radosz, A.
    Nasu, K.
    Powiązania:
    https://bibliotekanauki.pl/articles/1536487.pdf
    Data publikacji:
    2010-09
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    81.30.Hd
    61.66.-f
    Opis:
    We theoretically study possible domain-type collective dimerizations of graphite induced by inter-layer charge transfer excitations in the visible region. Using the semiempirical Brenner theory, we have calculated the adiabatic energy along the path that starts from original two distant graphite layers, but finally reaches the dimerized domain which consists of about 100 carbons with inter-layer σ-bonds. The energy barrier between this new domain and the starting graphite is shown to be of the order of 1 eV, being easily overcome by applying a few visible photons. We have also shown the optimal path of transformation via step by step increase of the domain size.
    Źródło:
    Acta Physica Polonica A; 2010, 118, 3; 500-506
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Photoinduced Conversion of Hybridization in Graphite
    Autorzy:
    Radosinski, L.
    Luty, T.
    Nasu, K.
    Ohnishi, H.
    Nishioka, K.
    Radosz, A.
    Wójt, D.
    Powiązania:
    https://bibliotekanauki.pl/articles/1490005.pdf
    Data publikacji:
    2012-02
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    81.30.Hd
    61.66.-f
    Opis:
    Recent experiments indicate that a photostimulated graphite with a femtosecond laser pulse results in the formation of a stable domain with sp^3 like interlayer bonds. By means of the energy barrier minimization and molecular dynamics using the empirical Brenner potential we study a geometrical structure of the new phase. We clarify proliferation of the initial domain and prove that the overall process is a multiphoton one. Furthermore, we present a model describing the initial transformation - an interlayer charge transfer resulting in the localization of an exciton-like state. The local density approximation electronic structure analysis reveals that the electronic state of the new phase is an insulator immersed in semimetal. We study by means of the long-range carbon bond order potential the effect of the existence of the new phase on the surrounding graphite and propose a new mid step structure on the path of a photoinduced graphite-diamond conversion.
    Źródło:
    Acta Physica Polonica A; 2012, 121, 2; 359-368
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    EPR Evidence for Thermally Excited Triplet States in Exinite, Vitrinite and Inertinite Separated from Bituminous Coal
    Autorzy:
    Słowik, G. P.
    Wojtowicz, W.
    Więckowski, A. B.
    Powiązania:
    https://bibliotekanauki.pl/articles/2043436.pdf
    Data publikacji:
    2005-07
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    61.66.Hq
    76.30.Rn
    87.64.Hd
    Opis:
    In this work we have made an electron spin resonance (EPR) study of macerals obtained from the lithotype clarain separated from Polish medium-rank coal (85.6 wt.% C). For three macerals:~exinite, vitrinite, and inertinite, the temperature dependence of intensity of EPR spectra in the temperature range of 100-373 K was investigated. The experimentally obtained EPR spectra of macerals were fitted by curves of the derivatives of the Gaussian and Lorentzian functions. The best fitting was obtained, when the experimental EPR spectra were assumed to be a superposition of three lines, for exinite and vitrinite - a broad Gaussian (G), a broad Lorentzian (L1) and a narrow Lorentzian (L3) line, but for inertinite of two lines - a narrow Lorentzian (L2) and a narrow Lorentzian (L3) line. The computer-assisted fitting has shown that each individual component line has similar values of resonance field, but different linewidths and amplitudes. The temperature dependence of line intensity I of the broad Gaussian (G) and narrow Lorentzian (L2 and L3) lines fulfils the Curie law in the form I=C/T or IT=C, whereas the broad Lorentzian (L1) line does not fulfil the Curie law. In the last case the temperature dependence of the Lorentzian (L1) component was fitted by the relation I=C/T+B/[T(3+exp(J/kT))] or IT=C+B/[3+exp(J/kT))], valid for thermally excited triplet states (S=1). For exinite and vitrinite the curves presenting the temperature dependence of the product IT versus temperature T were resolved into two curves, one for paramagnetic centres in the doublet state (S=1/2), and the other for paramagnetic centres in the thermally excited triplet state (S=1).
    Źródło:
    Acta Physica Polonica A; 2005, 108, 1; 171-176
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Kinetics of "order-order" Relaxations in Ni$\text{}_{3}$Al Studied by Computer Simulation
    Autorzy:
    Oramus, P.
    Kozubski, R.
    Cadeville, M. C.
    Pierron-Bohnes, V.
    Pfeiler, W.
    Powiązania:
    https://bibliotekanauki.pl/articles/2011010.pdf
    Data publikacji:
    1999-07
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    05.50.+q
    05.20.Dd
    66.30.-h
    81.30.Hd
    Opis:
    The experimental investigations of "order-order" kinetics in Ni$\text{}_{3}$ Al-based L1$\text{}_{2}$-ordered intermetallic compounds revealed the relaxation curves composed of two parallel processes considerably differing in relaxation rates. A simple Ising-type model based on a vacancy mechanism of atomic jumps was used to carry the Monte Carlo simulations of long-range-order relaxations in a binary A$\text{}_{3}$B system with L1$\text{}_{2}$-type superstructure. The simulated relaxation curves fitted weighted sums of two exponentials with significantly different relaxation times. It was found out that the fast relaxation process is controlled by the dynamics of the minority B-atom jumps.
    Źródło:
    Acta Physica Polonica A; 1999, 96, 1; 153-160
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
      Wyświetlanie 1-5 z 5

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