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Wyświetlanie 1-15 z 24
Tytuł:
Defect Mode in $LaB_{6}$
Autorzy:
Anisimov, M.
Bogach, A.
Glushkov, V.
Demishev, S.
Samarin, N.
Gavrilkin, S.
Mitsen, K.
Shitsevalova, N.
Levchenko, A.
Filippov, V.
Gabani, S.
Flachbart, K.
Sluchanko, N.
Powiązania:
https://bibliotekanauki.pl/articles/1371551.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
Opis:
The specific heat of high quality $La^{N}B_{6}$ (N=10, 11, natural) single crystals is investigated in a wide range of temperatures 2 - 300 K. The obtained data allow to estimate correctly (i) the electronic γ· T term of specific heat (γ ≈ 2.4 mJ/(mol·$K^{2}$)), (ii) the contribution from quasilocal vibrating mode of $La^{3+}$ ions ($Θ_{E}$ ≈ 150 - 152 K), (iii) the Debye-type term from rigid boron cages ($Θ_{D}$ ≈ 1160± 40 K). Our data also suggest an additional defect-mode component (iv) which may be attributed to a contribution of 1.5% boron vacancies in $LaB_{6}$. The obtained results may be interpreted in terms of formation of two level systems, which appear when $La^{3+}$ ions are displaced from their centrosymmetric positions in the cavities of rigid boron cages, apart from randomly distributed boron vacancies in the $LaB_{6}$ matrix.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 350-351
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Specific Heat and Magnetism of $LuFe_6Al_6$
Autorzy:
Svoboda, P.
Andreev, A.
Šantavá, E.
Šebek, J.
Powiązania:
https://bibliotekanauki.pl/articles/1813662.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.40.Cx
65.40.Ba
Opis:
Here we present the results of the zero-field specific heat study of the $LuFe_6Al_6$ single crystal. The specific heat data were analyzed as a sum of the phonon, electronic, and magnetic contributions, respectively. The analysis of the phonon part involves three acoustic and 36 optical branches, respectively, all of them corrected for the anharmonicity. The magnetic part of the specific heat was obtained by subtracting the electronic and the phonon part from the experimental specific heat and the magnetic entropy was calculated.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 307-310
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Lattice Heat Capacity in RTAl (R = Y, Lu;T = Ni, Cu, Pd) Compounds
Autorzy:
Daniel, P.
Javorský, P.
Prchal, J.
Daniš, S.
Šantavá, E.
Powiązania:
https://bibliotekanauki.pl/articles/1813674.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
75.40.Cx
Opis:
We present analysis of the specific heat of the RTAl (R = Y, Lu;T = Cu, Ni, Pd) compounds. We focus on the lattice contribution and analyze the dependence of all the characteristic parameters in the Debye and Einstein models on the atomic masses and interatomic distances.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 331-334
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Low Temperature Magnetic Ordering in NdAgAl₃
Autorzy:
Nallamuthu, S.
Džubinská, A.
Reiffers, M.
Nagalakshmi, R.
Powiązania:
https://bibliotekanauki.pl/articles/1032835.pdf
Data publikacji:
2017-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.70.Ch
65.40.Ba
Opis:
We present the detailed study of magnetic, thermodynamic, and transport properties of polycrystalline NdAgAl₃. The compound crystallizes in BaNiSn₃-type tetragonal structure with the space group I4mm. Magnetic, heat capacity and transport measurements indicate the possible antiferromagnetic nature of the ordering below 2 K. The compound shows the Schottky anomaly in heat capacity data. Magnetoresistance is negative at low temperature.
Źródło:
Acta Physica Polonica A; 2017, 131, 4; 1015-1017
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
New kinetic theory for absorption and emission rates of radiation and new equations for lattice and electronic heat capacities, enthalpies and entropies of solids: Application to copper
Autorzy:
Bozdoğan, A.
Powiązania:
https://bibliotekanauki.pl/articles/1057889.pdf
Data publikacji:
2017-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
44.40.+a
65.40.Ba
65.40.Gr
Opis:
New equations, which have analytical solutions, for lattice and electronic heat capacities, entropies and enthalpies at constant volume and constant pressure were derived by using kinetic theory, Kirchhoff and Stefan-Boltzmann laws and Wien radiation density equation. These equations were applied to the experimental constant volume heat capacity data of copper. The temperature Θ_{V} corresponding to 3R/2 was found to be 78.4 K for copper. Copper shows the dimensionality crossover from 3 to 2 at about 80 K. The Θ_{V}(T) is proportional to Debye temperature. The relationship between dimension and Θ_{V} was given. Temperature dependence of Debye temperature and non-monotonic behavior were discussed. The heat capacity and entropy values, predicted by the proposed models were compared with the values predicted by the Debye models. The results have shown that the proposed models fit the data better than the Debye models. Enthalpy equations derived in this study were compared with the polynomial model and a good fitting was obtained. The equation for the photon absorption equilibrium constant of copper was derived.
Źródło:
Acta Physica Polonica A; 2017, 131, 3; 519-526
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Ab Initio Study of the Mechanical, Thermal and Optoelectronic Properties of the Cubic CsBaF₃
Autorzy:
Harmel, M.
Khachai, H.
Haddou, A.
Khenata, R.
Murtaza, G.
Abbar, B.
Bin Omran, S.
Khalfa, M.
Powiązania:
https://bibliotekanauki.pl/articles/1402310.pdf
Data publikacji:
2015-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
62.20.de
65.40.Ba
65.40.De
Opis:
We have investigated the structural, elastic, electronic, optical and thermal properties of CsBaF₃ perovskite using the full-potential linearized augmented plane wave method within the generalized gradient approximation and the local density approximation. Moreover, the modified Becke-Johnson potential (TB-mBJ) was also applied to improve the electronic band structure calculations. The ground state properties such as lattice parameter, bulk modulus and its pressure derivative were calculated and the results are compared with the available theoretical data. The elastic properties such as elastic constants, anisotropy factor, shear modulus, Young's modulus and Poisson's ratio are obtained for the first time. Electronic and bonding properties are discussed from the calculations of band structure, density of states and electron charge density. The contribution of the different bands was analyzed from the total and partial density of states curves. The different interband transitions have been determined from the imaginary part of the dielectric function. The thermal effect on the volume, bulk modulus, heat capacities $C_V$ and the Debye temperature was predicted using the quasi-harmonic Debye model, in which the lattice vibrations are taken into account.
Źródło:
Acta Physica Polonica A; 2015, 128, 1; 34-42
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic specific heat of anion-radical salt [Ni(bipy)₃](TCNQ)₄·(CH₃)₂CO at very low temperatures
Autorzy:
Šoltésová, D.
Čižmár, E.
Vasylets, G.
Starodub, V.
Feher, A.
Powiązania:
https://bibliotekanauki.pl/articles/1053060.pdf
Data publikacji:
2017-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
75.30.Et
75.30.Gw
Opis:
Thermodynamic studies of the anion-radical salt system [Ni(bipy)₃](TCNQ)₄·(CH₃)₂CO, where TCNQ is 7,7',8,8'-tetracyano-quinodimethane, are reported. The anion-radical salt systems based on TCNQ belong to a material class in which the arrangement of the anion-radical salt has considerable impact on the charge transfer and magnetic properties. The crystal structure of the studied compound consists of [Ni(bipy)₃]⁺² cations containing Ni⁺² ions and four types of crystallographically independent anion-radicals TCNQ^{·-} (A, B, C and D). These TCNQ^{·-} radicals form two different types of TCNQ^{·-} stacks (AABB and CCDD), where a strong exchange interaction is expected. The temperature dependence of the specific heat of a single crystal was studied in magnetic fields up to 5 T and in the temperature range from 0.4 K to 30 K. The temperature dependence of specific heat displays a broad Schottky-like maximum above 0.4 K. Using a single-ion approximation, the analysis of the temperature dependence of the specific heat below 10 K yields values for the anisotropy parameters, D/k_{B}=-1.95 K and E/k_{B}=0.3 K. These results suggest that the observed maximum in the specific heat originates from Ni⁺² ions while the exchange interaction between the transition metal ions and the TCNQ is negligible.
Źródło:
Acta Physica Polonica A; 2017, 131, 4; 925-927
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Heat Capacity and Internal Pressure of Cyclopentanol at Pressures up to 100 MPa Determined by the Acoustic Method
Autorzy:
Dzida, M.
Powiązania:
https://bibliotekanauki.pl/articles/1811513.pdf
Data publikacji:
2008-12
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
82.30.Rs
62.50.-p
65.40.Ba
Opis:
Isobaric heat capacities and internal pressures of cyclopentanol at pressures up to 100 MPa and temperatures ranging from 293 to 318 K were determined by the acoustic method. The obtained results were compared with those of pentan-1-ol in order to study the influence of the molecular configurations comprising cyclic and normal-chain structures on pressure and temperature dependence of the thermodynamic properties. It was found that the temperature and pressure coefficients of internal pressure were sensitive to the structural organization of the liquid and reflected the character of the interactions.
Źródło:
Acta Physica Polonica A; 2008, 114, 6A; A-75-A-80
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Low Temperature Properties of the $Ce_{1-x}La_{x}NiAl_4$
Autorzy:
Toliński, T.
Kowalczyk, A.
Reiffers, M.
Šebek, J.
Šantavá, E.
Curlik, I.
Ilkovič, S.
Powiązania:
https://bibliotekanauki.pl/articles/1534742.pdf
Data publikacji:
2010-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.27.+a
65.40.Ba
75.30.Mb
Opis:
Measurements of the heat capacity in ultralow temperatures (down to 350 mK) have been carried out for $Ce_{1-x}La_{x}NiAl_4$. The paramagnetic behavior above about 30 K can be well described by the Curie-Weiss magnetic susceptibility. The undoped CeNiAl_4 compound is a known heavy fermion system with a large electronic specific heat coefficient (γ = 0.5 J $mol^{-1} K^{-2}$) and the Kondo temperature in the range 30-80 K. In the case of the $Ce_{0.8}La_{0.2}NiAl_4$ and $Ce_{0.6}La_{0.4}NiAl_4$ compounds a peak in C/T appears below 2 K, which is strongly damped by the magnetic field. It is probably connected with the Kondo and/or magnetic interactions and the electronic specific heat coefficient is 0.19 J $mol^{-1} K^{-2}$ (0.43 J $mol^{-1} K^{-2}$) for x = 0.2 (x = 0.4) at T → 0. The value determined above the peak, at temperature for which the magnetic field starts to decrease γ ( ≈ 3 K), is about 0.5 J $mol^{-1} K^{-2}$ and the effect of the magnetic field can be well analyzed in frames of the single-ion Kondo model.
Źródło:
Acta Physica Polonica A; 2010, 118, 5; 933-935
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Specific Heat and Magnetic Properties of Single-Crystalline $(Zn_{0.925}In_{0.054})[Cr_{1.84}In_{0.152}]Se_4$ Semiconductor
Autorzy:
Malicka, E.
Groń, T.
Pacyna, A.
Ślebarski, A.
Goraus, J.
Gągor, A.
Mydlarz, T.
Powiązania:
https://bibliotekanauki.pl/articles/1409656.pdf
Data publikacji:
2012-12
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
75.50.Ee
75.50.Pp
Opis:
An antiferromagnetic order with a Néel temperature $T_{N}$ = 17.5 K, a strong ferromagnetic exchange evidenced by a positive Curie-Weiss temperature $\Theta_{CW}$ = 77.3 K, the fuzzy peaks in the real component of susceptibility χ'(T) and the disappearance of the second critical field were established. The curvature of specific heat C(T) and C(T)/T in surrounding of $T_{N}$ indicated a broad peak, characteristic for the system with inhomogeneous magnetic state (spin-glass-like phase). The calculated magnetic entropy showed the value of S(T) ≈ 1 J/(mol K) which is extremely small; i.e., much lower than the magnetic contribution Rln(2S + 1) = 11.52 J/(mol K) calculated for the spin 3/2.
Źródło:
Acta Physica Polonica A; 2012, 122, 6; 1108-1110
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Specific Heat of the $Ce(Ni_{1 - x}Cu_{x})_4Mn$ Compounds
Autorzy:
Synoradzki, K.
Toliński, T.
Powiązania:
https://bibliotekanauki.pl/articles/1427043.pdf
Data publikacji:
2012-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
75.50.Cc
75.50.Lk
Opis:
Specific heat of the $Ce(Ni_{1 - x}Cu_{x})_4Mn$ compounds has been studied. The samples are prepared by induction melting and it is found, based on the X-ray diffraction, that all the compounds keep the $CaCu_5$-type structure. This series exhibits a transition between the ferromagnetically ordered $CeNi_4Mn$ and the spin-glass $CeCu_4Mn$ compounds, which is well visible in the measurements of the ac susceptibility peak as a function of the magnetic field frequency and in the magnetization relaxation. In the present research we explore the behavior of the specific heat for various x. The changes of the electronic specific heat coefficient γ are determined by analysis of the low temperature part of the $C_{p}//T(T^2)$ dependence. We also observe that the magnetic phase transition is only detectable in the specific heat signal after extraction of the magnetic contribution of the Mn atoms. This is carried out by subtraction of the specific heat of the reference sample.
Źródło:
Acta Physica Polonica A; 2012, 121, 5-6; 1079-1081
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Specific Heat of $YbNi_4Si$ Compound
Autorzy:
Falkowski, M.
Kowalczyk, A.
Toliński, T.
Powiązania:
https://bibliotekanauki.pl/articles/1813487.pdf
Data publikacji:
2008-02
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
82.80.Pv
65.40.Ba
75.20.Hr
Opis:
The specific heat of $YbNi_4Si$ has been analyzed considering the electronic contribution and the lattice contributions in frames of the Debye model. Based on the specific heat measurements, the electronic specific heat coefficient γ = 25 mJ $mol^{-1} K^{-2}$ and the Debye temperature $θ_D$ = 320 K were derived. This small value shows that $YbNi_4Si$ cannot be classified as a heavy fermion system. These studies are completed by magnetic susceptibility, X-ray photoemission spectroscopy, and electrical resistivity.
Źródło:
Acta Physica Polonica A; 2008, 113, 2; 641-644
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Heat Capacity of Heavy Fermion Compound $CeCu_4Ga$ in High Magnetic Fields
Autorzy:
Kowalczyk, A.
Toliński, T.
Reiffers, M.
Zapotoková, M.
Falkowski, M.
Gažo, E.
Powiązania:
https://bibliotekanauki.pl/articles/1810399.pdf
Data publikacji:
2009-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.Ba
71.20.Eh
71.27.+a
Opis:
The heat capacity in the applied magnetic field up to 9 T, susceptibility and magnetization of polycrystalline $CeCu_{4}Ga$ are presented. Magnetic ordering was not observed down to 2 K. For temperature T < 200 K a Curie-Weiss behavior is observable giving an effective magnetic moment $μ_\text{eff}$ =2.53 $μ_{B}$/f.u. The experimental value of $μ_\text{eff}$ is close to the calculated one for a free $Ce^{3+}$ ion ($μ_\text{eff}$ = 2.54 $μ_{B}$/f.u.), thus indicating the presence of well localized magnetic moments carried by the stable $Ce^{3+}$ ions. At low temperatures the electronic heat capacity coefficient value depends strongly on the temperature range used for the extrapolation and applied magnetic field. We observe a typical heavy fermion behavior with γ value of about 380 mJ $\text{mol}^{-1} K^{-2}$ obtained from extrapolation to T = 0 K of the temperature range above 7 K. However, extrapolation of the lowest temperatures range yields the γ value of 3.3 J $\text{mol}^{-1} K^{-2}$.
Źródło:
Acta Physica Polonica A; 2009, 115, 1; 123-125
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Ab Initio Studies on Structural, Elastic, Thermodynamic and Electronic Properties of FeCrAs under Pressures
Autorzy:
He, De-Chun
Peng, Yong
He, Yong-Wei
Powiązania:
https://bibliotekanauki.pl/articles/1400506.pdf
Data publikacji:
2015-06
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
62.20.de
65.40.Ba
65.40.De
72.15.-v
Opis:
The structural, elastic, thermodynamic and electronic properties of nonmetallic metal FeCrAs are studied within density function perturbation theory. The thermodynamic properties of FeCrAs were deduced based on phonon frequencies within the framework of the quasiharmonic approximation. The calculated elastic modulus under various pressures indicates that FeCrAs is mechanically stable under pressure. The pressure-dependence of bulk and shear modulus, transverse and longitudinal sound velocities V (i.e. $V_{S}$ and $V_{L}$), elastic Debye temperature $\Theta_{E}$ of FeCrAs have also been investigated. The calculated values of B/G indicate that FeCrAs presents high ductility under pressure. However, it is interesting that the value of B/G reaches a maximum under 40 GPa and almost remains unchanged when the pressure is above 70 GPa. The calculations show that the heat capacity $C_{V}$ of this material is close to the Dulong-Petit limit 3R (about 224.61 J $mol^{-1} K^{-1}$) at high temperature regime. The analysis of electronic properties find that as the pressure increases, the absolute value of charge for As and Fe atom increases while Cr remains nearly a constant, indicating that the mechanic properties of FeCrAs under pressure should be mostly attributed to the interaction between Fe and As atoms.
Źródło:
Acta Physica Polonica A; 2015, 127, 6; 1637-1644
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
The Solid State Polymorphism and Dynamics of 2,3-Dimethylbutan-2-ol (2,3-DM-2-B)
Autorzy:
Juszyńska, E.
Massalska-Arodź, M.
Zieliński, P.
Krawczyk, J.
Powiązania:
https://bibliotekanauki.pl/articles/1418234.pdf
Data publikacji:
2012-10
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
65.40.-b
65.40.Ba
66.30.hp
77.22.Gm
Opis:
In the paper we present adiabatic calorimetry and dielectric spectroscopy results for 2,3-dimethylbutan-2-ol (2,3-DM-2-B), one of the isomers of neohexanol. For 2,3-DM-2-B we have detected the following phase transitions: C2 (249.8 K) → C1 (262 K) → Is. No glass phase was found. In both crystalline phases C2 and C1 three relaxation processes were detected. These processes are discussed in relation to the calorimetric studies.
Źródło:
Acta Physica Polonica A; 2012, 122, 4; 693-697
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Wyświetlanie 1-15 z 24

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