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Wyświetlanie 1-15 z 15
Tytuł:
Some Comments on p-Ps and Density Parameter
Autorzy:
Goworek, T.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/1933488.pdf
Data publikacji:
1995-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
36.10.Dr
Opis:
The constraint-free analysis of several representative positron lifetime spectra was performed with the resolution time of 144 ps. The role of p-Ps parameters in understanding of the positronium structure in solids is discussed.
Źródło:
Acta Physica Polonica A; 1995, 88, 1; 135-138
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron Porosimetry Studies of Template Removal from As-Synthesized MCM-41 Silica
Autorzy:
Zaleski, R.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/1812554.pdf
Data publikacji:
2008-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
78.70.Bj
36.10.Dr
61.43.Gt
81.07.-b
Opis:
The course of template removal from MCM-41 pores was investigated by positron annihilation lifetime spectroscopy. Two methods of removal were the object of interest: a decarbonisation after standard calcination procedure and a novel procedure - pyrolysis in vacuum. The shapes of positron lifetime spectra of decarbonised sample are determined by positronium quenching caused by presence of carbon deposit on the surface. Positron annihilation lifetime spectroscopy allows also monitoring the evolution of empty space inside pores. During pyrolysis no conductive carbon is produced, so consecutive stages of template material transformation are easy to observe. In the case of pyrolysis the effect of pore emptying is obtained at temperature 500 K, lower comparing to calcination and decarbonisation (820 K).
Źródło:
Acta Physica Polonica A; 2008, 113, 5; 1543-1550
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Electron traps in long-chain alkanes
Autorzy:
Pietrow, M.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/146299.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
PALS
positron annihilation
electron traps
quenching by light
Opis:
Positron lifetime spectra in long-chain alkanes were measured at various wavelengths of light illuminating the samples as a function of temperature, storage time. It was found that in n-alkanes with carbon chain longer than 30 atoms two kinds of electron traps exist; the depth of shallower of them is less than 0.52 eV. They are discharged already at a temperature of 120 K.
Źródło:
Nukleonika; 2010, 55, 1; 51-55
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Vapour Absorption in Melamine-Formaldehyde Resin
Autorzy:
Wawryszczuk, J.
Ciesielski, K.
Goworek, J.
Powiązania:
https://bibliotekanauki.pl/articles/2025738.pdf
Data publikacji:
2001
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
78.70.Bj
36.10.Dr
61.41.+e
66.30.-h
Opis:
The effects of vapour absorption on positron annihilation in cross-linked polymer were investigated. Contrary to linear polymers, absorption of vapour in cross-linked resin leads to the shortening of o-Ps lifetime. In vacuum absorbed molecules diffuse out. At room temperature desorption of hexane and hexanol is not complete; full elimination of absorbed molecules requires sample temperature increase.
Źródło:
Acta Physica Polonica A; 2001, 99, 3-4; 523-528
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Influence of Temperature and Pressure on the Free Volume in Thermo-Shrunken Polyethylene by Positron Annihilation
Autorzy:
Danch, A.
Osoba, W.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/1812484.pdf
Data publikacji:
2008-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.60.+z
78.70.Bj
Opis:
Positron lifetime measurements were performed as a function of temperature and pressure for thermo-shrunken polyethylene. Mean volume of free volume cavities in the investigated polymer was estimated from the results of the measurements. This mean volume turned out to be the smooth function of temperature (from room temperature to 8.5 K) and high pressure (from 0.1 MPa to about 500 MPa). The effect of trapping of the free electrons produced during positron irradiation was observed at low temperature.
Źródło:
Acta Physica Polonica A; 2008, 113, 5; 1307-1313
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positronium Formation in Solid Long-Chain Alkanes
Autorzy:
Zaleski, R.
Wawryszczuk, J.
Goworek, T.
Powiązania:
https://bibliotekanauki.pl/articles/2042188.pdf
Data publikacji:
2005-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
36.10.Dr
78.70.Bj
Opis:
This paper represents a fragment of systematic studies on positron annihilation in solid saturated hydrocarbons (alkanes, paraffins) from C$\text{}_{17}$H$\text{}_{36}$ to C$\text{}_{30}$H$\text{}_{62}$. The Tao-Eldrup model and its extensions allow to identify the places in the crystalline structure where positronium is trapped, and estimate respective trap sizes. In the rigid phase I positronium locates mainly in two-dimensional empty spaces between the lamellae of crystal structure. Additional free volumes exist in high temperature phases due to appearance of n-alkane conformers representing a non-planar molecule distortion. The rise of ortho-positronium intensity with the sample irradiation dose, which was seen earlier in polymers, is observed also in n-alkanes. One can find similarities between the ortho-positronium annihilation in crystalline alkanes and polymers, like exponential character of that rise, and the trap bleaching by illumination. It confirms the same origin of the intensity growth, i.e. the accumulation of trapped electrons. Two kinds of electron traps were found. The time constant of electron accumulation in the traps depends on the carbon chain length and varies with temperature in different way for even- and odd-numbered alkanes.
Źródło:
Acta Physica Polonica A; 2005, 107, 4; 635-641
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Three-Quantum Annihilation in Porous Vycor Glass
Autorzy:
Jasińska, B.
Wawryszczuk, J.
Zaleski, R.
Powiązania:
https://bibliotekanauki.pl/articles/2043332.pdf
Data publikacji:
2005-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
36.10.Dr
78.70.Bj
Opis:
Three methods of determination of 3γ o-Ps decay intensity are compared. The estimate of 3γ fraction obtained from classical lifetime measurements can be distorted due to a higher absorption of theγ quanta from the continuous spectrum of three-quantum decay, compared to two-quantum one.
Źródło:
Acta Physica Polonica A; 2005, 107, 5; 821-825
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Pressure Effects in ortho-Positronium Annihilation
Autorzy:
Goworek, T.
Wawryszczuk, J.
Zaleski, R.
Powiązania:
https://bibliotekanauki.pl/articles/2042179.pdf
Data publikacji:
2005-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
36.10.Dr
78.70.Bj
Opis:
A short review of experiments concerning the influence of high pressure on positron annihilation in molecular solids is given. To this kind of experiments belong e.g. pressure inhibition of positronium formation, pressure induced phase transitions, and free volume swelling in the media intercalated by high pressure gas.
Źródło:
Acta Physica Polonica A; 2005, 107, 4; 608-614
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positrons in naphthalene : critical remarks on the relation between o-Ps lifetime and void size
Autorzy:
Goworek, T.
Zgardzińska, B.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/148003.pdf
Data publikacji:
2013
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
high pressure
naphthalene
positronium quenching
free volume
Opis:
Lowering the temperature or applying high pressure leads to elimination of positronium component in the e+ lifetime spectrum in solid naphthalene. Disappearance of positronium means reaching the free volume size limit at which there is no energy level in the potential well. It allows to estimate that size, which is found inconsistent with predictions of the popular Tao-Eldrup model. The range of applicability of that model is discussed. The dependence of the free e+ decay constant on pressure indicates that positronium is formed not only in the blob processes, but during the whole free positron life. The lifetime of free positrons begins to rise with temperature earlier than Ps intensity.
Źródło:
Nukleonika; 2013, 58, 1; 183-187
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Distortion of the Positron Lifetime Spectra in BaF$\text{}_{2}$ Spectrometers
Autorzy:
Goworek, T.
Górniak, W.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/1858021.pdf
Data publikacji:
1993-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
06.50.Dc
07.85.+n
Opis:
High efficiency of BaF$\text{}_{2}$ scintillators creates the risk of distortion of the positron lifetime distributions due to summing and backscattering. In the 180° geometry it leads to the appearance of a spurious shortlived component.
Źródło:
Acta Physica Polonica A; 1993, 83, 3; 307-311
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Positron annihilation lifetime spectroscopy study of thermal processing and rehydration of dry leek (Allium porrum L.)
Autorzy:
Zaleski, R.
Wawryszczuk, J.
Sobczak, K.
Powiązania:
https://bibliotekanauki.pl/articles/146309.pdf
Data publikacji:
2010
Wydawca:
Instytut Chemii i Techniki Jądrowej
Tematy:
positron annihilation
lifetime spectroscopy
food processing
rehydration
leek (Allium porrum L.)
Opis:
New application of positron annihilation lifetime spectroscopy (PALS) to development of food processing techniques is tested. Dehydrated leeks were an object of the study. Three experiments were performed consisting of evacuating air and volatile compounds from the sample, applying thermal treatment and rehydrating the sample. Distinct changes in positron lifetime spectra allowed the monitoring of alterations in the sample structure. The most likely origin of the particular components present in the spectra was able to be proposed from these data. Changes of the components were ascribed to the various processes occurring in the samples.
Źródło:
Nukleonika; 2010, 55, 1; 73-78
0029-5922
1508-5791
Pojawia się w:
Nukleonika
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Ortho-Positronium in Some n-Alkanes; Influence of Temperature and Pressure
Autorzy:
Zgardzińska, B.
Pietrow, M.
Goworek, T.
Wawryszczuk, J.
Powiązania:
https://bibliotekanauki.pl/articles/2047166.pdf
Data publikacji:
2006-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
36.10.Dr
61.80.Fe
71.60.+z
78.70.Bj
Opis:
Positron lifetime spectra were measured for a series of odd-numbered n-alkanes from C$\text{}_{11}$H$\text{}_{24}$ to C$\text{}_{19}$H$\text{}_{40}$ as a function of temperature and pressure. The ortho-Ps lifetimes in the rotator phase and the increase in intensity at the transition to that phase can be explained by location of Ps in the vicinity of kink-type conformers. The relation between o-Ps lifetime and molecule length can be described in the framework of extended Tao-Eldrup model. One can eliminate the effect of intensity rise in time by sample illumination or by application of high pressure. A decrease in temperature by 1 K is equivalent to an increase in pressure by about 4 MPa.
Źródło:
Acta Physica Polonica A; 2006, 110, 5; 747-753
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Testing the Extended Tao-Eldrup Model. Silica Gels Produced with Polymer Template
Autorzy:
Śniegocka, M.
Jasińska, B.
Wawryszczuk, J.
Zaleski, R.
Deryło-Marczewska, A.
Skrzypek, I.
Powiązania:
https://bibliotekanauki.pl/articles/2043364.pdf
Data publikacji:
2005-05
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
78.70.Bj
61.43.Gt
Opis:
The temperature dependence of o-Ps lifetime in the pores calculated from extended Tao-Eldrup model was compared to the experimental data, collected for a set of silica gels synthesized using the polymer template technique. For the sample with average pore radii 2.0 nm rather good agreement between the model and experiment was found. For the sample with narrow pores (near 1.0 nm) the lifetime spectrum was complex. Except the range of highest temperatures the lifetimes are far from model calculations.
Źródło:
Acta Physica Polonica A; 2005, 107, 5; 868-873
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
An Attempt to Produce the Implanted $\text{}^{22}$Na Source for Positron Spectrometry
Autorzy:
Latuszyński, A.
Yushkevich, Yu. V.
Bystrov, V. A.
Misak, R.
Wawryszczuk, J.
Goworek, T.
Powiązania:
https://bibliotekanauki.pl/articles/1929102.pdf
Data publikacji:
1993-03
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
28.60.+s
29.25.Rm
Opis:
Preliminary results of $\text{}^{22}$Na implantation into the metal foils in order to produce the positron source for annihilation experiments are presented.
Źródło:
Acta Physica Polonica A; 1993, 83, 3; 345-348
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
The Temperature and Pressure Dependence of the Free Volume in Fluoroelastomers from PALS and PVT Experiments
Autorzy:
Dlubek, G.
Sen Gupta, A.
Wawryszczuk, J.
Kilburn, D.
Pionteck, J.
Krause-Rehberg, R.
Goworek, T.
Alam, M. A.
Kaspar, H.
Lochhaas, K. H.
Powiązania:
https://bibliotekanauki.pl/articles/2042202.pdf
Data publikacji:
2005-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
61.41.+e
78.70.-g
Opis:
Positron lifetime and pressure-volume-temperature experiments were performed as function of T (100-485 K) and P (10$\text{}^{-5}$ Pa-500 MPa) on a fluoroelastomer. From positron annihilation lifetime spectroscopy, analyzed with LT9.0 assuming a dispersion in the e$\text{}^{+}$ (τ$\text{}_{2}$) and o-Ps (τ$\text{}_{3}$) lifetime, the mean, 〈v$\text{}_{h}$〉, and the width (standard deviation), σ$\text{}_{h}$, of the hole size distribution were calculated. The pressure-volume-temperature data were analyzed using the Simha-Somcynsky hole-lattice theory to estimate the specific hole free volume V$\text{}_{f}$. From a comparison of V$\text{}_{f}$ with 〈v$\text{}_{h}$〉 the specific hole number, N'$\text{}_{h}$, is estimated. The data from thermal expansion and pressure experiments show complete agreement when taking into account the compressibility of the occupied volume.
Źródło:
Acta Physica Polonica A; 2005, 107, 4; 685-689
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
    Wyświetlanie 1-15 z 15

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