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Tytuł:
Magnetism in $NdMnO_{3+δ}$ Studied by the Single Crystal Neutron Diffraction
Autorzy:
Mihalik, M.
Maťaš, S.
Vavra, M.
Powiązania:
https://bibliotekanauki.pl/articles/1368766.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.20.-g
75.30.-m
75.50.Gg
Opis:
We present the single crystal neutron diffraction experiment performed on the $NdMnO_{3+δ}$ compound. The aim of the experiment was to study/revisit the magnetic structure of the compound. We have confirmed the ordering of Mn sublattice below $T_{N}$=85.5 K and confirmed that the Nd sublattice orders below $T_{1}$ ≈ 20 K with Nd moments aligned parallel to the b-axis.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 284-285
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Valence Band and Core Levels of $Ce_5Ni_2Si_3$ Crystal Studied by X-ray Photoemission Spectroscopy
Autorzy:
Toliński, T.
Kowalczyk, A.
Chełkowska, G.
Mihalik, M.
Timko, M.
Powiązania:
https://bibliotekanauki.pl/articles/1813673.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.20.Eh
82.80.Pv
Opis:
The crystal of $Ce_5Ni_2Si_3$ was prepared by the Czochralski method. The X-ray photoemission spectroscopy was measured for the valence band and the core levels. Based on the Ce(3d) doublet and its satellites a small value of the hybridization parameter of the f-states with the conduction electrons Δ=4 meV and the f-occupancy $n_f$ close to 1 were found. X-ray photoemission spectroscopy shows that the region between 0 and 3 eV is predominated by the Ni(3d) and Ce(4f) peaks. Some features of the multiplet structure of the Ce(4f) states are also visible close to the Fermi level.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 327-330
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Anisotropy of Susceptibility and Optical investigation of the Antiferromagnetic phase Transition in U$\text{}_{1-x}$Ce$\text{}_{x}$Ru$\text{}_{2}$Si$\text{}_{2}$
Autorzy:
Mihalik, M.
Maťaš, S.
Macko, D.
Timko, M.
Menovsky, A. A.
Powiązania:
https://bibliotekanauki.pl/articles/1955512.pdf
Data publikacji:
1997-02
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.30.Hb
75.20.Hr
72.15.-v
Opis:
Temperature dependence of magnetic susceptibility of U$\text{}_{1-x}$Ce$\text{}_{x}$Ru $\text{}_{2}$Si$\text{}_{2}$ single crystals (x=0, 0.025, 0.05, 0.075) has been studied at temperatures from 4.2 K up to room temperature and in magnetic fields applied along and perpendicular to the c-axis. The attention was paid to anomalies connected with the antiferromagnetic phase transition, which are present in crystals with x≤0.05. Far-infrared measurements of U$\text{}_{0.99}$Ce$\text{}_{0.01}$ Ru$\text{}_{2}$Si$\text{}_{2}$ single crystal have been studied for the first time. The measurements support the assumption that the origin of magnetic ordering in U$\text{}_{0.99}$Ce$\text{}_{0.01}$Ru$\text{}_{2}$Si$\text{}_{2}$ is the same as in heavy-fermion superconductor URu$\text{}_{2}$Si$\text{}_{2}$ and can be interpreted as being due to a spin-density-wave gap.
Źródło:
Acta Physica Polonica A; 1997, 91, 2; 351-354
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Effect of Pressure on Magnetic Properties of Hexacyanochromates
Autorzy:
Mitróvá, Z.
Maťaš, S.
Mihalik, M.
Zentková, M.
Arnold, Z.
Kamarád, J.
Powiązania:
https://bibliotekanauki.pl/articles/1813813.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.30.Cr
75.50.Ee
75.50.Gg
75.50.Xx
Opis:
We present the study of pressure effect on magnetic properties of $TM^{2+}_3[Cr^{III}(CN)_6]_2 \cdot nH_2O$ ferrimagnets and ferromagnets (TM = Cr and Co) under pressures up to 0.9 GPa. Applied pressure strengthens super-exchange interaction in $Cr^{2+}$-prussian blue analogues with dominant antiferromagnetic interaction $J_{AF}$ leading to increase in the Curie temperature $T_C$ (ΔT_c/Δp = 29.0 K/GPa) and reduces $T_C$ of $Co^{2+}$-prussian blue analogues with dominant ferromagnetic interaction $J_F$ (Δ$T_c$/Δp = -1.8 K/GPa). The rise of $J_{AF}$ interaction is attributed to the enhanced value of the single electron overlapping integral S. On the other hand, the applied pressure slightly affects bonding angles between magnetic ions mediated by the cyano-bridge and reduces the strength of magnetic coupling. Changes of the magnetization curve with pressure can be attributed to changes of magnetic anisotropy. The reduction of magnetization with pressure observed on $Cr^{2+}$-prussian blue analogues can be explained by pressure induced transition from $Cr^{2+}$ high spin state to $Cr^{2+}$ low spin state. All pressure induced changes are reversible.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 469-472
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic Properties of $(Cu_{x}Mn_{1-x})_3[Cr(CN)_6]_2$ · $zH_2O$ Complexes
Autorzy:
Vavra, M.
Antoňák, M.
Jagličić, Z.
Mihalik, M.
Csach, K.
Zentková, M.
Powiązania:
https://bibliotekanauki.pl/articles/1535120.pdf
Data publikacji:
2010-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.30.Kz
75.30.Cr
Opis:
Magnetization measurements were performed on the $(Cu_{x}Mn_{1-x})_3[Cr(CN)_6]_2$ · $zH_2O$ molecule-based magnets where x=0.0, 0.2, 0.25, 0.3, 0.35 0.4, 0.6, 0.8 and 1.0. Both the Curie temperature and saturated magnetization at first decrease with increasing value of x reaching the minimal value of $T_{C}$ = 49.7 K and 0.17 $μ_{B}$ for x=0.2 and then increase with substitution. The pronounced hysteretic behavior between zero-field cooled and field cooled regimes was observed for all samples. Magnetization changes the sign of magnetic polarization in zero-field cooled magnetization curve at the compensation temperature $T_\text{comp}$ = 16 K for sample with x = 0.4. Our results indicate that the system behaves as mixed-ferri-ferromagnetic system.
Źródło:
Acta Physica Polonica A; 2010, 118, 5; 998-999
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic Properties of $La_{0.8}K_{0.2}MnO_{3}$ Nanoparticles
Autorzy:
Mihalik, M.
Zentková, M.
Briančin, J.
Fitta, M.
Lazúrová, J.
Vavra, M.
Powiązania:
https://bibliotekanauki.pl/articles/1371270.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.50.-y
75.47.Lx
75.30.-m
75.30.Kz
Opis:
Magnetic properties of $La_{0.8}K_{0.2}MnO_{3}$ have been studied on nanoparticles prepared by glycine-nitrate method. Crystal structure and particles size were modified by heat treatment. Crystal structure changes from orthorhombic (space group Pbma) to rhombohedral (space group R-3c) after annealing at 600°C/2 hours. The average size of particle varies with annealing from about 30 nm to 135 nm. The Curie temperature $T_{C}$ and the saturated magnetization $μ_{s}$ increase with annealing. The exchange bias effect was observed on samples with particles size smaller than 60 nm.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 312-313
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Effect of the Jahn-Teller Distortion on Double Exchange Interaction in $La_{0.8}K_{0.2}MnO_3$ Nanoparticles
Autorzy:
Mihalik, M.
Zentková, M.
Vavra, M.
Mihalik Jr., M.
Lazúrová, J.
Girman, V.
Konieczny, P.
Fitta, M.
Il'kovič, S.
Powiązania:
https://bibliotekanauki.pl/articles/1398285.pdf
Data publikacji:
2017-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.50.-y
75.47.Lx
75.30.-m
75.30.Kz
Opis:
Electric resistance and effect of hydrostatic pressure on magnetic properties has been studied on the $La_{0.8}K_{0.2}MnO_3$ nanoparticles. Magnetic phase transition is affected by pressure only slightly, the Curie temperature $T_{C}$ decreases with the rate of -1.02 K/GPa, on samples with orthorhombic structure where the Jahn-Teller distortion of lattice is large. On the other hand, $T_{C}$ increases with the rate of 20.1 K/GPa on samples with rhombohedral structure, where the Jahn-Teller distortion of lattice is absent. Insulator type of electrical resistance is characteristic feature of sample with large Jahn-Teller distortion of lattice and insulator-metal transition was observed on samples where the Jahn-Teller distortion is negligible. Our results are in line with theoretical calculation predicting that double exchange interaction is suppressed by the Jahn-Teller distortion.
Źródło:
Acta Physica Polonica A; 2017, 131, 4; 875-877
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Exchange bias effect in NdFeO₃ system of nanoparticles
Autorzy:
Vavra, M.
Zentková, M.
Mihalik, M.
Mihalik Jr., M.
Lazúrová, J.
Girman, V.
Perovic, M.
Kusigerski, V.
Roupcova, P.
Jaglicic, Z.
Powiązania:
https://bibliotekanauki.pl/articles/1054801.pdf
Data publikacji:
2017-04
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.47.Lx
75.50.Tt
75.70.Rf
75.60.Jk
Opis:
We study the effect of nanometric size on the crystal structure, magnetic environment of iron and magnetization in NdFeO₃ system of nanoparticles. The average particle size of NdFeO₃ nanoparticles increases with annealing at 600°C from about 15 nm to 40 nm. The smallest particles on annealed sample have size approximately 30 nm and typically have character of single crystalline samples. All samples adopt orthorhombic crystal structure, space group Pnma with lattice parameters a =5.5817 Å, b=7.7663 Å and c =5.456 Å for as prepared sample. The presence of superparamagnetic particles was indicated by the Mössbauer measurements. The reduction of dimensionality induces a decrease of T_{N1} from 691 K to 544 K. The shift of magnetic hysteresis loop in vertical and horizontal direction was observed at low temperatures after cooling in magnetic field. We attribute such behaviour to exchange bias effect and discuss in the frame of core-shell model.
Źródło:
Acta Physica Polonica A; 2017, 131, 4; 869-871
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic Properties of $La_{0.85}Ag_{0.15}MnO_{3}$ Nano-Powders Under Pressure
Autorzy:
Antoňák, M.
Mihalik, M.
Zentková, M.
Vavra, M.
Lazúrová, J.
Fitta, M.
Balanda, M.
Powiązania:
https://bibliotekanauki.pl/articles/1369756.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.50.-y
75.50.Tt
75.47.Lx
75.30.Kz
Opis:
In our paper we present effect of pressure on magnetic properties of $La_{0.85}Ag_{0.15}MnO_{3}$ nanopowders prepared by glycine-nitrate method. The particle size and crystal structure were modified by heat treatment. The average size of particle varies from about 25 nm for as prepared sample to 60 nm for annealed sample. Crystal structure changes from orthorhombic to rhombohedral after annealing at 600 °C/2 hours. The Curie temperature increases with annealing and is more than doubled after annealing at 600 °C/2 hours. The exchange bias phenomenon was observed in samples with orthorhombic crystal structure with average particle size of about 25 nm. Pressure effect on the Curie temperature $T_{C}$, saturated magnetization $μ_{s}$ and exchange bias field $H_{E}$ is negligible in this case. In the case of the samples with rhombohedral structure, $T_{C}$, $μ_{s}$ and remnant magnetization $μ_{r}$ increase with pressure; the coercive field decreases with pressure.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 296-297
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic Properties of Milled and Thermal Relaxed YBa$\text{}_{2}$ (Cu$\text{}_{1-x}$Fe$\text{}_{x}$)$\text{}_{3}$O$\text{}_{y}$
Autorzy:
Timko, M.
Kováč, J.
Sargánková, I.
Zentková, M.
Mihalik, M.
Maťaš, S.
Čiasnohová, A.
Powiązania:
https://bibliotekanauki.pl/articles/1955517.pdf
Data publikacji:
1997-02
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
74.90.+n
74.10.+v
74.70.-b
Opis:
The influence of the mechanical milling and subsequent thermal relaxation on magnetic and superconducting behaviour of YBa$\text{}_{2}$(Cu$\text{}_{1-x}$Fe $\text{}_{x}$)$\text{}_{3}$O$\text{}_{y}$ system has been studied. Two methods of heat treatment were used: Set I - slow cooling from 980°C in flowing O$\text{}_{2}$ and Set II - reducing at 770°C in flowing Ar$\text{}_{2}$ followed by reoxidation in flowing O$\text{}_{2}$ below 400°C. The transition to superconductivity, diamagnetic response, critical current density and the effective magnetic moment in the normal state have been estimated. Our measurements indicate that the reducing atmosphere preparation is less detrimental on superconducting properties. The results are discussed in terms of occupancy Cu sites by Fe and redistribution of oxygen atoms.
Źródło:
Acta Physica Polonica A; 1997, 91, 2; 355-358
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic Properties of $NdFe_{0.9}Mn_{0.1}O_{3}$
Autorzy:
Zentková, M.
Lazúrová, J.
Kováč, J.
Mihalik, M.
Briančin, J.
Fitta, M.
Kusigerski, V.
Powiązania:
https://bibliotekanauki.pl/articles/1371226.pdf
Data publikacji:
2014-07
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.50.-y
75.47.Lx
75.30.-m
75.30.Kz
75.30.Et
75.30.Cr
Opis:
In our paper we study effect of Mn for Fe substitution on magnetic properties of $NdFe_{x-1}Mn_{x}O_{3}$ compounds for x=0 and 0.1, which have been grown by the OFZ technique. The Néel temperature decreases from $T_{N1}$=691 K to $T_{N1}$=621 K, and the anomaly in AC susceptibility, related to spin reorientation, vanishes with Mn substitution. Low temperature heat capacity measurement for sample with x=0.1 revealed that substitution of Mn for Fe shifts a Schottky-type anomaly at $T_{sh}$ to higher temperatures. Another anomaly is generated by doping at $T_{max}$=11 K. The anomaly is smeared out by magnetic field, confirming its magnetic origin.
Źródło:
Acta Physica Polonica A; 2014, 126, 1; 306-307
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetism of Nanoparticle $La_{0.7}Ca_{0.3}Mn_{0.7}Fe_{0.3}O_3$ under Applied Hydrostatic Pressure
Autorzy:
Kusigerski, V.
Perovic, M.
Mrakovic, A.
Blanusa, J.
Mihalik, M.
Zentkova, M.
Spasojevic, V.
Powiązania:
https://bibliotekanauki.pl/articles/1534028.pdf
Data publikacji:
2010-11
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
75.50.Tt
75.75.-c
81.07.Bc
Opis:
Nanoparticle $La_{0.7}Ca_{0.3}Mn_{0.7}Fe_{0.3}O_3$ with the average particle size of 10 nm was mechanochemically synthesized in the single-step procedure. Temperature and field dependences of magnetization were recorded under both ambient and applied hydrostatic pressure up to 0.47 GPa. At ambient pressure, two magnetic transition points were observed: one of the spin-glass like type at the temperature $T_{f}$ ≈ 34 K, and ferro-to-paramagnet transition at $T_{C}$ ≈ 51 K. Under the applied pressure magnetic parameters gradually changed: (i) both $T_{C}$ and $T_{f}$ were lowered with the increase in pressure; (ii) both high field magnetization $M_{5T}$ and remanent magnetization $M_{Rem}$ decreased with pressure; (iii) coercivity $H_{C}$ increased with pressure. The obtained results show that magnetism of a nanoparticle system with high degree of intrinsic disorder diminishes with the applied pressure that is in compliance with the effect of the increased cationic disorder ("internal pressure") in bulk manganites.
Źródło:
Acta Physica Polonica A; 2010, 118, 5; 811-812
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Magnetic and Transport Properties of $La_{0.67}Pb_{0.33}(Mn_{1-x}Co_x)O_3$
Autorzy:
Mihalik, M.
Kavečanský, V.
Maťaš, S.
Zentková, M.
Ammer, J.
Kellner, K.
Gritzner, G.
Powiązania:
https://bibliotekanauki.pl/articles/1813631.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.30.+h
72.80.Ga
75.20.Hr
75.30.Et
75.30.Vn
Opis:
Detailed studies of temperature dependences of magnetization, AC susceptibility and electrical resistance were performed on $La_{0.67}Pb_{0.33}(Mn_{1-x}Co_x)O_3$ ceramics with x = 0.01 and 0.1. Typical features of both compounds are the hysteretic behavior between the zero-field-cooled magnetization regime and the field-cooled magnetization regime, a very weak field dependence of a maximum in zero-field-cooled magnetization and practically no frequency dependence of the peak in AC susceptibility χ"(T). Anomalies in the electrical resistance connected with the ferromagnetic transition at $T_C$, the insulator-metal transitions at $T_p$ and the re-entrant metal-isolator transition at T* are field dependent pointing to magnetic origin of these transitions. Colossal magnetoresistance was observed in both compounds.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 251-254
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
Electronic States of $UNi_2$ from Photoemission Spectroscopy
Autorzy:
Zalecki, R.
Kołodziejczyk, A.
Kim-Ngan, N.
Adamska, A.
Kowalczyk, A.
Toliński, T.
Mihalik, M.
Powiązania:
https://bibliotekanauki.pl/articles/1813761.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
71.20.Lp
79.60.Bm
71.15.Ap
Opis:
We measured the angle-resolved ultraviolet and X-ray photoemission spectra of $UNi_2$ single crystal. The valence band angle-resolved ultraviolet photoemission spectra were compared to the accessible band structure calculations. For $UNi_2$ the lowest binding energy strong emission at about -0.1 eV comes from U 5f states and overlaps with the Fermi edge. A small feature at -0.6 eV was ascribed also to U 5f electrons with more localised character. The higher-energy two-peak structure at about -1.2 eV and -2.1 eV comes from Ni 3d states. X-ray photoemission spectroscopy shows the standard two-line spin-orbit splitting of the Ni 2p states and of the U 4f states. Some hybridisation of the Ni 3d and U 5f state was observed in the spectra. The pronounced satellites to the Ni 2p and 3p states, associated with the on-site Coulomb repulsion and other electron correlation energies, were observed.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 407-412
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Tytuł:
$\text{}^1H$ NMR on $(Ni_xMn_{1-x})_3[Cr(CN)_6]_2 \cdot nH_2O$
Autorzy:
Bokor, M.
Tompa, K.
Kiss, L.
Zentková, M.
Zentko, A.
Mihalik, M.
Maťaš, S.
Mitróová, Z.
Powiązania:
https://bibliotekanauki.pl/articles/1813831.pdf
Data publikacji:
2008-01
Wydawca:
Polska Akademia Nauk. Instytut Fizyki PAN
Tematy:
72.80.Ga
75.50.Xx
76.60.Lz
Opis:
We report on $\text{}^1H$ NMR of $(Ni_xMn_{1-x})3[Cr(CN)_6]_2 \cdot 15H_2O$ hexacyanochromates, where x changes from 0 to 1. The decay time constants of the free induction decay signals described by an effective spin-spin relaxation time $T_{2eff}$ obtained from M(t) = $M_0 \text{exp}(t//T_{2eff})$ decrease as the local magnetic moments increase produced by the magnetic transition metal ions at the sites of the resonant $\text{}^1H$ nuclei. The recovery of the magnetization in the spin-lattice relaxation time $(T_1)$ experiments was single-exponential.
Źródło:
Acta Physica Polonica A; 2008, 113, 1; 485-488
0587-4246
1898-794X
Pojawia się w:
Acta Physica Polonica A
Dostawca treści:
Biblioteka Nauki
Artykuł
Wyświetlanie 1-15 z 23

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