- Tytuł:
- Valence Band of $Ce_2Co_{0.8}Si_{3.2}$ and $Ce_2RhSi_3$ Studied by Resonant Photoemission Spectroscopy and FPLO Calculations
- Autorzy:
-
Starowicz, P.
Kurleto, R.
Goraus, J.
Walczak, Ł.
Penc, B.
Adell, J.
Szlawska, M.
Kaczorowski, D.
Szytuła, A. - Powiązania:
- https://bibliotekanauki.pl/articles/1374249.pdf
- Data publikacji:
- 2014-10
- Wydawca:
- Polska Akademia Nauk. Instytut Fizyki PAN
- Tematy:
-
71.27.+a
75.30.Mb
71.20.Eh
74.25.Jb - Opis:
- This work presents studies of the valence band of two Kondo lattice systems: $Ce_2Co_{0.8}Si_{3.2}$, which is paramagnetic with the Kondo temperature $T_{K}$ ≈50 K and $Ce_2RhSi_3$, which is antiferromagnetic below $T_{N}$=4.5 K and exhibits $T_{K}$ ≈9 K. The photoemission spectra, which are obtained with photon energy tuned to Ce 4d-4f resonance, reveal a Kondo peak at the Fermi energy $(E_{F})$, its spin-orbit splitting partner at 0.24 eV and a broad maximum related to Ce $f^0$ final state. The spectra indicate that Kondo peak has a higher intensity for $Ce_2Co_{0.8}Si_{3.2}$. The off-resonance photoemission data reveal that a maximum in the 3d electron density of states is shifted towards $E_{F}$ for $Ce_2Co_{0.8}Si_{3.2}$ as compared to $Ce_2RhSi_3$. Full-potential local-orbital calculations were realized with local spin density approach +U approach for 213 stoichiometry. They show that a higher density of states near $E_{F}$ is observed for $Ce_2CoSi_3$. The calculations also reveal the existing tendencies for antiferromagnetic and ferromagnetic ground states in a case of $Ce_2RhSi_3$ and $Ce_2CoSi_3$, respectively.
- Źródło:
-
Acta Physica Polonica A; 2014, 126, 4a; A-144-A-147
0587-4246
1898-794X - Pojawia się w:
- Acta Physica Polonica A
- Dostawca treści:
- Biblioteka Nauki
Artykuł