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    Tytuł:
    Effect of acid buffering capacity on the remobilization of heavy metals in sewage sludge barrier for tailings
    Autorzy:
    Chen, Y.
    Zhang, H.
    Ju, Y.
    Powiązania:
    https://bibliotekanauki.pl/articles/205048.pdf
    Data publikacji:
    2018
    Wydawca:
    Polska Akademia Nauk. Czytelnia Czasopism PAN
    Tematy:
    sewage sludge
    heavy metals
    acid mine drainage
    acid buffering capacity
    remobilization
    Opis:
    Remobilization of heavy metals from the bottom liner system due to the seepage of acid mine drainage (AMD) is an important concern in the long-term management of tailing impoundment. Titration tests were carried out to evaluate the acid buffering capacity (ABC) of sewage sludge and to investigate its effect on the remobilization of heavy metals. Test results demonstrate that the ABC increases with solid/liquid ratio and anaerobic incubation time and it is mainly attributed to the abundant organic matters contained and increasing carbonate loads. The added heavy metals (Zn, Pb, and Cu) were well immobilized during the anaerobic incubation stage but were released out dramatically during the acidification especially when pH drops below 6.0 because of dissolution of carbonates and cation exchange of clay minerals. The calculated results, from a simplified model, indicate that high levels of remobilization of heavy metals are not expected during the typical management time because of the high ABC of compacted sewage sludge barrier. These results support that sewage sludge is a suitable bottom liner material for the management of AMD from tailings.
    Źródło:
    Archives of Environmental Protection; 2018, 44, 2; 62-72
    2083-4772
    2083-4810
    Pojawia się w:
    Archives of Environmental Protection
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Aluminum-Doped Zinc Oxide Thin Films Prepared by Sol-Gel and~RF Magnetron Sputtering
    Autorzy:
    Wu, G.
    Chen, Y.
    Lu, H.
    Powiązania:
    https://bibliotekanauki.pl/articles/1504062.pdf
    Data publikacji:
    2011-07
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    81.15.Cd
    82.70.Gg
    77.55.hf
    Opis:
    Zinc oxide (ZnO) thin films have become technologically important materials due to their wide range of electrical and optical properties. The characteristics can be further adjusted by adequate doping processes. In this paper, aluminum-doped zinc oxide thin films have been prepared on glass substrates using a sol-gel route and the radio-frequency magnetron sputtering process. The stoichiometry could be easily adjusted by controlling the nanosized precursor concentration and the thickness by dip-coating cycles. On the other hand, the mixed $N_2O//Ar$ plasma gas provided adequate N doping for the RF sputtering process. The results showed the low electrical resistivity of 21.5 Ω cm with the carrier concentration of - 3.21 × $10^{18} cm^{-3}$ for the n-type aluminium-doped zinc oxide film. They were 34.2 Ω cm and + 9.68 × $10^{16} cm^{-3}$ for the p-type aluminium-doped zinc oxide film. The optical transmittance has been as high as 85-90% in the 400-900 nm wavelength range. The aluminium-doped zinc oxide (2 at.% Al) films exhibited the hexagonal wurzite structure with (002) preferred crystal orientation. The electrical characteristics were depicted by the gradual increase in N and NO that occupy the oxygen vacancies.
    Źródło:
    Acta Physica Polonica A; 2011, 120, 1; 149-152
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Spatiotemporal analysis of air quality and its relationship with meteorological factors in the Yangtze River Delta
    Autorzy:
    Li, Y.
    Chen, Y.
    Karimian, H.
    Tao, T.
    Powiązania:
    https://bibliotekanauki.pl/articles/1192096.pdf
    Data publikacji:
    2020
    Wydawca:
    Uniwersytet Warmińsko-Mazurski w Olsztynie / Polskie Towarzystwo Magnezologiczne im. Prof. Juliana Aleksandrowicza
    Tematy:
    YRD
    air quality index
    meteorological elements
    correlation analysis
    air pollution
    spatial analysis
    Opis:
    Air quality is closely related to people’s health and life. In addition to being directly affected by social activities and atmospheric emissions, the impacts of meteorological factors are also significant. Based on daily Air Quality Index (AQI) data and various meteorological parameters in the Yangtze River Delta (YRD), this paper summarized the spatiotemporal evolution characteristics of AQI over YRD, and quantitatively analyzed the contribution of different meteorological elements to air quality. We also evaluated different spatial interpolation methods to produce surface distribution of AQI, and noted that the Ordinary Kriging outperformed other methods. The spatial distribution of AQI in YRD showed seasonal and annual variations. However, the days with AQI over 100 (level ii) were mostly observed in winter. Generally, more severe air pollution was observed in the northern part of YRD than in the southern ones, for example the air quality of the Ningbo metropolitan area was the best, while in Hefei it was the worst. It was found that meteorological parameters have spatially varying effects on AQI. For instance, pressure has a significant positive effect on AQI, and others showed negative correlations. We also predicted AQI by exploiting different machine learning-based models. Through model comparison, it was found that the Autoregressive Integrated Moving Average Model – ARIMA (0,1,2) has higher prediction accuracy for AQI than Multiple Linear Regression (MLR). The findings of this research can be used in future forecasting of air pollution, and also in air pollution controlling programs.
    Źródło:
    Journal of Elementology; 2020, 25, 3; 1059-1075
    1644-2296
    Pojawia się w:
    Journal of Elementology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Catalytic decomposition of toluene over La1-xSr xMnO3/palygorskite synthesized catalysts
    Autorzy:
    Song, L.
    Chen, T.
    Chen, D.
    Chen, Y.
    Xie, J.
    Liu, H.
    Powiązania:
    https://bibliotekanauki.pl/articles/207996.pdf
    Data publikacji:
    2013
    Wydawca:
    Politechnika Wrocławska. Oficyna Wydawnicza Politechniki Wrocławskiej
    Tematy:
    catalysts
    manganese
    manganese oxide
    toluene
    transmission electron microscopy
    X ray diffraction
    Palygorskite
    katalizatory
    mangan
    tlenek manganu
    toluen
    transmisyjna mikroskopia elektronowa
    dyfrakcja promieniowania rentgenowskiego
    Opis:
    Palygorskite (PG) supported La1-xSrxMnO3 catalysts were fabricated by copreripitation. The catalysts were characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), specific surface area (SSA) and H2 temperature programmed reduction (H 2-TPR). Catalytic activity for VOCs was examined by using toluene as a model compound. The results show that the surface area as well as mechanical strength of catalysts increase substantially after catalysts loaded in PG. XRD patterns show that after calcination at 700 0C, PG as a support in 9% LaMn03/PG and 9% La0.7Sr0.3MnO3/PG was transformed into amorphous phase and the morphology was not destroyed. It was well established that the main reductive components are factually Mn(III) or Mn(IV) oxides in catalysts based on the results of TPR. It was also found that Mn(IV) increases while Mn(III) reduces responding with the increasing amount of Sr. Toluene conversion rate of as-preparedμ% La1-xSr xMnO3/PG increases with the increasing values of x and μ when x=0-0.3 and μ = 3-9%. Toluene can be converted completely at 285 0C by 9% La0.7Sr0.3MnO3/PG catalyst while no significant change was observed after addition on the doping and loading amount of Sr. During a 100 h stability experiment of 9% La 0.7Sr0.3MnO3/PG catalyst, toluene removal was found to be above 95%.
    Źródło:
    Environment Protection Engineering; 2013, 39, 3; 31-42
    0324-8828
    Pojawia się w:
    Environment Protection Engineering
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Flotation behavior and adsorption mechanism of sodium lauroamphoacetate to cassiterite
    Autorzy:
    Chen, Y.
    Lv, H.
    Tong, X.
    Xie, X.
    Powiązania:
    https://bibliotekanauki.pl/articles/109885.pdf
    Data publikacji:
    2018
    Wydawca:
    Politechnika Wrocławska. Oficyna Wydawnicza Politechniki Wrocławskiej
    Tematy:
    sodium lauroamphoacetate
    flotation behavior
    adsorption mechanism
    cassiterite
    Opis:
    The flotation behavior and adsorption mechanism of cassiterite using sodium lauroamphoacetate (SLA) as a collector were investigated by adsorption tests, micro-flotation tests, zeta potential measurements, Fourier transform infrared spectroscopy (FTIR) and X-ray photoelectron spectroscopy (XPS) analysis. Adsorption test results indicated that the adsorption of SLA on the cassiterite surface increased continually with the increase of SLA concentration. Micro-flotation test results demonstrated that SLA had a stronger collecting ability to cassiterite than salicylhydroxamic acid (SHA) and sodium oleate (NaOL) in the pH range of 2-12, and showed a higher selectivity in the separation of cassiterite-quartz than in cassiterite-clinochlore. The zeta potential measurement results indicated that the isoelectric point (IEP) of cassiterite minerals changed from pH 3.9 to 3.4, suggesting the adsorption of SLA on cassiterite surface. The FTIR spectra and XPS analysis further confirmed that SLA chemically adsorbed on cassiterite surface.
    Źródło:
    Physicochemical Problems of Mineral Processing; 2018, 54, 2; 386-394
    1643-1049
    2084-4735
    Pojawia się w:
    Physicochemical Problems of Mineral Processing
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Experimental study on triboelectrostatic beneficiation of wet fly ash using Microwave Heating
    Autorzy:
    Li, H.
    Chen, Y.
    Zhang, X.
    Zhao, Y.
    Tao, Y.
    Li, C.
    He, X.
    Powiązania:
    https://bibliotekanauki.pl/articles/110399.pdf
    Data publikacji:
    2016
    Wydawca:
    Politechnika Wrocławska. Oficyna Wydawnicza Politechniki Wrocławskiej
    Tematy:
    wet fly ash
    triboelectrostatic beneficiation
    microwave heating
    efficiency
    Opis:
    Triboelectrostatic beneficiation, as a physical method, of fly ash cannot only meet the technical requirements of fly ash application but also recycle of an unburned carbon as a useful energy source. The aim of this study was to investigate the feasibility of improving efficiency of triboelectrostatic beneficiation of wet fly ash using microwave heating. The wet fly ash with different moisture contents had an average loss-on-ignition of 12.56%. The fly ash samples were heated in a microwave oven before the experiments. The experimental conditions were electric field voltage of 40 kV and air flux ranging from 12 to 30 m3/h. The influence of the microwave heating on the wet fly ash triboelectrostatic beneficiation was discussed under the conditions of different microwave intensity and irradiation time. The results indicated that the removal rate and recycle rate of the unburned carbon showed a significant increase performance as the wet fly ash was processed by the microwave heating which was attributed to changes of moisture contents and dielectric constants caused by the microwave heating. The feasibility had been verified according to the experimental study on fly ash with different moisture contents. It can be concluded that the microwave heating process was efficiently applied for the wet fly ash triboelectrostatic beneficiation.
    Źródło:
    Physicochemical Problems of Mineral Processing; 2016, 52, 1; 328-341
    1643-1049
    2084-4735
    Pojawia się w:
    Physicochemical Problems of Mineral Processing
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Interface Engineering in Heteroepitaxy
    Autorzy:
    Hong, S. K.
    Chen, Y.
    Ko, H. J.
    Yao, T.
    Powiązania:
    https://bibliotekanauki.pl/articles/2035571.pdf
    Data publikacji:
    2002
    Wydawca:
    Polska Akademia Nauk. Instytut Fizyki PAN
    Tematy:
    68.35.-p
    68.35.Dv
    81.15.-z
    81.15.Hi
    81.10.Aj
    Opis:
    We report the importance of interface engineering in heteroepitaxy with examples of plasma-assisted molecular beam epitaxial ZnO growths on (0001) sapphire substrates and on (0001) GaN/sapphire templates, whose interfaces are engineered to improve and to control properties of ZnO films. The growth of rocksalt structure MgO buffer on Al$\text{}_{2}$O$\text{}_{3}$ (0001) is developed for ZnO epitaxy. By employing the MgO buffer layer, the formation of 30$\text{}^{o}$ rotated mixed domains is prohibited and two-dimensional layer-by-layer growth of ZnO on sapphire substrate is achieved. High-resolution X-ray diffraction reveals the superior improvement in a crystal quality of ZnO films with an MgO buffer. Polarity of wurtzite structure ZnO films on Ga-polar GaN/sapphire templates is controlled by changing interface structures. By forming a single crystalline, monoclinic Ga$\text{}_{2}$O$\text{}_{3}$ interfacial layer between GaN and ZnO through O-plasma pre-exposure on the Ga-polar GaN surface, O-polar ZnO films are grown. By forming the ZnO/GaN heterointerface without an interfacial layer through the Zn pre-exposure on the Ga-polar GaN surface, Zn-polar ZnO films are grown.
    Źródło:
    Acta Physica Polonica A; 2002, 102, 4-5; 541-554
    0587-4246
    1898-794X
    Pojawia się w:
    Acta Physica Polonica A
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Study on electric spring control method considering noncritical load voltage constraint
    Autorzy:
    Chen, Y.
    Ma, G.
    Xu, U.
    Zhang, H.
    Ju, R.
    Powiązania:
    https://bibliotekanauki.pl/articles/140516.pdf
    Data publikacji:
    2018
    Wydawca:
    Polska Akademia Nauk. Czytelnia Czasopism PAN
    Tematy:
    electric spring
    noncritical load
    voltage excursion
    reactive power compensation
    Opis:
    With the increasing penetration rate of grid-connected renewable energy generation, the problem of grid voltage excursion becomes an important issue that needs to be solved urgently. As a new type of voltage regulation control method, electric spring (ES) can alleviate the fluctuations of renewable energy output effectively. In this paper, the background and basic principle of the electric spring are introduced firstly. Then, considering the influence of an electric spring on noncritical load voltage, noncritical loads are classified reasonably, and based on the electric spring phasor diagram, the control method to meet the noncritical load voltage constraint is proposed. This control method can meet the requirements of voltage excursions of different kinds of noncritical load, increase the connection capacity of the noncritical load and improve the voltage stabilization capacity of the electric spring. Finally, through the simulation case, the feasibility and validity of electric spring theory and the proposed control method are verified.
    Źródło:
    Archives of Electrical Engineering; 2018, 67, 4; 709-724
    1427-4221
    2300-2506
    Pojawia się w:
    Archives of Electrical Engineering
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    A Facile Synthesis of 3,3'-Dinitro-5,5'-diamino-bi-1,2,4-triazole and a Study of Its Thermal Decomposition
    Autorzy:
    Ma, Q.
    Lu, H.
    Qu, Y.
    Liao, L.
    Li, J.
    Fan, G.
    Chen, Y.
    Powiązania:
    https://bibliotekanauki.pl/articles/358272.pdf
    Data publikacji:
    2017
    Wydawca:
    Sieć Badawcza Łukasiewicz - Instytut Przemysłu Organicznego
    Tematy:
    3,3’-dinitro-5,5’-diamino-bi-1,2,4-triazole
    facile synthesis
    DSC-TG
    RSFTIR
    TG-IR
    thermolysis
    Opis:
    3,3’-Dinitro-5,5’-diamino-bi-1,2,4-triazole (DABNT) was synthesized by a facile method and its crystalline density was determined as 1.839 g·cm−3 at 293(2) K by X-ray diffraction. Its thermal decomposition kinetics and mechanism were studied by means of differential scanning calorimetry-thermogravimetry (DCS-TG), in situ thermolysis by rapid-scan Fourier transform infrared spectroscopy (RSFTIR) and simultaneous TG-IR technology. The results showed that the apparent activation energies obtained by the Kissinger, Ozawa and Starink methods were 122.9 kJ·mol−1, 123.2 kJ·mol−1 and 123.5 kJ·mol−1, respectively. The thermodynamic parameters of ΔS≠, ΔH≠ and ΔG≠ were −37.5 J·K−1·mol−1, 118.4 kJ·mol−1 and 138.7 kJ·mol−1, respectively. The decomposition reaction process of DABNT starts with the transformation from a primary amine to a secondary amine and then the loss of one nitro-group from the DABNT structure. Gaseous products, such as N2O and H2O, were detected from decomposition in the range of 50-300 °C. Density functional theory (DFT) calculations were further employed to illustrate the decomposition mechanism. The above-mentioned information on the synthesis and thermal behaviour is quite useful for the scale-up and evaluation of the thermal safety of DABNT.
    Źródło:
    Central European Journal of Energetic Materials; 2017, 14, 2; 281-295
    1733-7178
    Pojawia się w:
    Central European Journal of Energetic Materials
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Preliminary results of spatial distribution of uranium and thorium in soil profi les near a uranium industrial site, Guangdong province, China
    Autorzy:
    Wang, J.
    Liu, J.
    Chen, Y.
    Song, G.
    Chen, D.
    Xiao, T.
    Li, H.
    Wang, C.
    Jiang, F.
    Powiązania:
    https://bibliotekanauki.pl/articles/146530.pdf
    Data publikacji:
    2016
    Wydawca:
    Instytut Chemii i Techniki Jądrowej
    Tematy:
    spatial distribution
    thorium
    uranium
    U/Th ratio
    Opis:
    Four soil profiles were collected from locations with different distances (5, 50, 250 and 1000 m) from a uranium mill tailings dam, Guangdong province, China, to investigate the pollution status of the soil in mining/ milling-related areas based on the contents of uranium (U) and thorium (Th), thus to understand the impacts of uranium industrial activities to the surroundings. The U and Th concentrations were determined by inductively coupled plasma mass spectrometry (ICP-MS) after conventional HF-HNO3-HClO4 digestion procedures. The results indicate that the soils within 50 m from uranium tailing were severely contaminated; those in 250 and 1000 m soil samples were observed to be with local background level even though these in 250 m had slightly higher U/Th ratios. Uranium concentrations varied from 5.50 ± 0.27 to 160.55 ± 8.03 mg/kg, with maximum values recorded in an intermediate layer of the 5-m distance soil profile. In comparison, the concentration of Th ranged from 6.02 ± 0.30 to 84.71 ± 4.24 mg/kg, with maximum values observed in the top layer of the 1000-m distance soil profile. The U/Th ratio varied from 0.15 to 11.99 compared with 0.20, 0.22 and 0.26 of the average for Guangdong province, national China and the world, respectively. The mean U/Th of four soil profiles showed a reduction with distance from the uranium mill tailing dam, suggesting the relatively large magnitude of uranium elevation in soils within limited distances.
    Źródło:
    Nukleonika; 2016, 61, 3; 367-371
    0029-5922
    1508-5791
    Pojawia się w:
    Nukleonika
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
      Wyświetlanie 1-10 z 10

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