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    Wyświetlanie 1-14 z 14
    Tytuł:
    Dry and steam reforming of methane. Comparison and analysis of recently investigated catalytic materials. A short review.
    Autorzy:
    Summa, Paulina
    Samojeden, Bogdan
    Motak, Monika
    Powiązania:
    https://bibliotekanauki.pl/articles/779028.pdf
    Data publikacji:
    2019
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    dry methane reforming
    steam methane
    reforming
    nickel catalyst
    hydrotalcite
    Opis:
    In order to produce valuable syngas, industrial processes of dry reforming of methane and steam reforming of methane must be further developed. This paper is focused on reviewing recently examined catalysts, supporting the mentioned technologies. In both processes the most popular active material choice is usually nickel, due to its good availability. On the other hand, noble metals, such as ruthenium, rhodium or platinum, provide better performance, however the solution is not cost-effective. Materials used as a support influence the catalytic activity. Oxides with basic properties, such as MgO, Al2 O3 , CeO2 , are frequently used as carriers. One of the most promising materials for reforming of methane technologies are hydrotalcites, due to adjustable composition, acid-base properties and possibility of incorporation of various metals and complexes.
    Źródło:
    Polish Journal of Chemical Technology; 2019, 21, 2; 31-37
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Bromine catalyst for the methane to methyl bisulfate reaction
    Autorzy:
    Michalkiewicz, B.
    Balcer, S.
    Powiązania:
    https://bibliotekanauki.pl/articles/778989.pdf
    Data publikacji:
    2012
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    methane
    methyl bisulfate
    methanol
    KBr
    Opis:
    A catalytic system KBr – oleum is effective at catalyzing the selective oxidation of methane to methanol via. methyl bisulfate. The infl uences of methane pressure, sulfur trioxide and temperature on turnover frequency were investigated.
    Źródło:
    Polish Journal of Chemical Technology; 2012, 14, 4; 19-21
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Bio-methanization of organic fraction from municipal solid waste: temperature effects
    Autorzy:
    Fernández-Rodríguez, J.
    Pérez, M.
    Romero, L. I.
    Powiązania:
    https://bibliotekanauki.pl/articles/779264.pdf
    Data publikacji:
    2013
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    anaerobic digestion
    OFMSW
    mesophilic
    thermophilic
    methane
    Opis:
    The main objective of this study was to analyse the development of dry anaerobic digestion process of OFMSW in batch reactors under two temperature ranges, thermophilic (55°C) and mesophilic (35°C). The experimental results lead to the conclusion that the thermophilic range has a greater rate of hydrolysis and is therefore more effective to degrade wastes, shortening the overall operating time. For example, the hydrolytic step in the thermophilic (T) process lasted an average of 8 days versus 14 days in the mesophilic (M) range. The methanogenic phase lasted for 18 and 29 days in the T and M processes, respectively. The mesophilic range showed higher removal of the organic effluent but with greater uptime requirements. Moreover, the thermophilic range showed greater productivities than the mesophilic range, and the productivities were approximately doubled in terms of the produced biogas from a given amount of consumed organic matter.
    Źródło:
    Polish Journal of Chemical Technology; 2013, 15, 2; 99-106
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Homogeneous catalytic systems for selective oxidation of methane: state of the art
    Autorzy:
    Balcer, S.
    Powiązania:
    https://bibliotekanauki.pl/articles/777855.pdf
    Data publikacji:
    2015
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    alkane functionalization
    methane
    methanol
    catalytic systems
    homogeneous catalytic systems
    Opis:
    Homogeneous catalysts for methane oxidation are of a particular interest from scientific and economic points of view. The results show a great potential for activation and functionalization of CH bonds of unreactive methane. There are still gaps in the knowledge of how to rationally design catalysts for this process. In this paper state-of-the-art. in methane oxidation homogenous catalysis is presented.
    Źródło:
    Polish Journal of Chemical Technology; 2015, 17, 3; 52-61
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Simulation of SOFCs based power generation system using Aspen
    Autorzy:
    Pianko-Oprych, P.
    Palus, M.
    Powiązania:
    https://bibliotekanauki.pl/articles/778251.pdf
    Data publikacji:
    2017
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    Solid Oxide Fuel Cell system
    modelling
    methane
    reforming
    CPOx
    Opis:
    This study presents a thermodynamic Aspen simulation model for Solid Oxide Fuel Cells, SOFCs, based power generation system. In the first step, a steady-state SOFCs system model was developed. The model includes the electrochemistry and the diffusion phenomena. The electrochemical model gives good agreement with experimental data in a wide operating range. Then, a parametric study has been conducted to estimate effects of the oxygen to carbon ratio, O/C, on reformer temperature, fuel cell temperature, fuel utilization, overall fuel cell performance, and the results are discussed in this paper. In the second step, a dynamic analysis of SOFCs characteristic has been developed. The aim of dynamic modelling was to find the response of the system against the fuel utilization and the O/C ratio variations. From the simulations, it was concluded that both developed models in the steady and dynamic state were reasonably accurate and can be used for system level optimization studies of the SOFC based power generation system.
    Źródło:
    Polish Journal of Chemical Technology; 2017, 19, 4; 8-15
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Localization of fugitive methane emission from natural gas distribution network of Titas Gas
    Autorzy:
    Mandal, P. C.
    Morshed, S. M.
    Powiązania:
    https://bibliotekanauki.pl/articles/778196.pdf
    Data publikacji:
    2017
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    fugitive emission
    methane release
    gas leakage
    leak constant
    climate mitigation
    Opis:
    The aim of this paper is to localize the fugitive leaks from the above ground facilities of the existing system of Titas Gas (TG) after developing mathematical model for fugitive emission. Soap screening techniques and Gasurveyor 500 series instrument were used in this study for detecting potential leaks. Leaked gas was quantified using either Hi-Flow gas sampler or bagging measurements system. The results show that the respective potential gas leaking point of City Gate Station (CGS), commercial Regulating and Metering Station (RMS), industrial RMS, residential RMS and Town Bordering Station (TBS)/ District Regulating Station (DRS) are scrubber dump valve (average leak rate 217.00 L/min), insulating point (average leak rate 4.04 L/min), tube fitting connector (average leak rate 8.00 L/min), connector (average leak rate 1.55 L/min) and pressure relief valve (average leak rate 437.92 L/min). Fugitive methane emission can be reduced by stopping leaks of fittings or components having high KLeak  value.
    Źródło:
    Polish Journal of Chemical Technology; 2017, 19, 1; 127-131
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Methane fermentation of poultry slaughterhouse waste
    Autorzy:
    Wymysłowski, M.
    Łuczak, M.
    Zawadzka, A.
    Imbierowicz, M.
    Chacuk, A.
    Powiązania:
    https://bibliotekanauki.pl/articles/779316.pdf
    Data publikacji:
    2010
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    fermentacja metanowa
    odpady drobiowe
    termohydroliza
    methane fermentation
    poultry waste
    thermohydrolysis
    Opis:
    One of the alternative methods for the treatment of animal by-products is their utilization in biological processes with a simultaneous production of energy-rich biogas. The results of the investigations of methane fermentation of animal waste are discussed in the study. The methane fermentation was carried out at 35°C. The substrates used in the experiments included poultry heads and muscle tissue. Furthermore, the fermentation residues subjected previously to hydrothermal processing were used as a substrate. The suspension of those substrates in the initial concentration range from 1 g TOC/dm3 to 11 g TOC/dm3 was used in the process. Additionally, the effect of the preliminary stage of hydrothermal substrate processing on methane fermentation efficiency was assessed. Poultry waste was subjected to thermohydrolysis at the temperature from 100°C to 300°C and pressure up to 9.0 MPa. The efficiency of the methane fermentation was estimated on the basis of biogas generated in the process. The biogas production was between 0.17 Ndm3/g TOC and 1.53 Ndm3/g TOC. In the case of poultry heads, a beneficial impact of hydrothermal processing at the temperatures from 100°C to 175°C was confirmed. For poultry meat the preliminary thermohydrolysis brought about a decrease of methane fraction in the biogas evolved. The preliminary hydrothermal processing made it possible to meet the requirements of legal regulations for the hygienization of by-products of animal origin. The obtained results allowed us to identify conditions under which the methane fermentation was carried out and which ensured a high level of methanization.
    Źródło:
    Polish Journal of Chemical Technology; 2010, 12, 3; 15-18
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Catalysts for the utilization of methane from the coal mine ventilation air
    Autorzy:
    Stasińska, B.
    Machocki, A.
    Powiązania:
    https://bibliotekanauki.pl/articles/777952.pdf
    Data publikacji:
    2007
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    powietrze wentylacyjne
    kopalnia węgla
    metan
    utylizacja metanu
    katalityczne utlenianie metanu
    katalizator tlenkowy
    katalizator palladowy
    coal mine ventilation air
    utilization of methane
    catalytic oxidation of methane
    oxide catalysts
    palladium catalysts
    Opis:
    The paper indicates coal mines as the source of permanent emission of low-concentrated gases, which have increased the greenhouse effect. This paper proposes the catalytic oxidation of methane as the solution to the problem of methane utilization when its concentration in the air is insufficient for flame combustion. The studies which have been conducted for many years enabled finding the active oxide and metallic catalytic systems for the reaction of methane oxidation. For the utilization of gases with low-concentrated methane, using the low-temperature catalysts, especially palladium catalysts, seems to he economically well-justified. Depending on technological solutions it can be considered as the method for methane utilization or as an environmentally friendly way for the generation of electric and thermal energy.
    Źródło:
    Polish Journal of Chemical Technology; 2007, 9, 3; 29-32
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Assessment of the possibility of the methane to methanol transformation
    Autorzy:
    Michalkiewicz, B.
    Powiązania:
    https://bibliotekanauki.pl/articles/779700.pdf
    Data publikacji:
    2008
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    metan
    metanol
    wodorosiarczan metylu
    wykres Sankeya
    bilans masy
    methane
    methanol
    methyl bisulphate
    Sankey diagram
    mass balance
    Opis:
    The methane to methanol conversion via esterification is an interesting method which makes it possible to eliminate the otherwise necessary phase of obtaining synthesis gas. On the basis of laboratory investigations mass balances for this process were determined. Preliminary assessment of the way of conducting the process and possibilities of practical applications of this technology was also made. It was pointed out that regardless of any possible modifications of methane to methanol conversion via esterification redundant sulfuric acid will always be produced during ester hydrolysis. Production of methanol from methane using this method can only be done when it is combined with producing other substances, which needs using H2SO4.
    Źródło:
    Polish Journal of Chemical Technology; 2008, 10, 2; 20-26
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    The simplex optimization for high porous carbons preparation
    Autorzy:
    Sreńscek-Nazzal, J.
    Michalkiewicz, B.
    Powiązania:
    https://bibliotekanauki.pl/articles/779821.pdf
    Data publikacji:
    2011
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    węgiel porowaty
    aktywacja chemiczna
    metoda simplex
    adsorpcja metanu
    porous carbon
    chemical activation
    simplex method
    methane adsorption
    Opis:
    The microporous carbon materials were prepared by chemical activation of Polish coal with potassium hydroxide using the simplex design method for planning the experiments. The experimental parameters were varied to identify the optimum conditions. Coal can be an excellent starting material for the preparation of high porous carbons for natural gas storage. The porosity of the resultant carbons was characterized by nitrogen adsorption (-196oC). Methane adsorption was investigated in a volumetric laboratory installation at range pressures from 1 to 3.5 MPa (25oC). The best results of methane storage capacity (557 cm3 . g-1) were obtained when using an impregnation ratio 3.41/1 KOH/precursor and temperature at 592oC, (SLANG = 2091 m2 . g-1). The parameters of the preparation of high porosity and high methane adsorption carbon were determined by a fast and simple method.
    Źródło:
    Polish Journal of Chemical Technology; 2011, 13, 4; 63-70
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Catalityc removal of nitrogen oxide from combustion gases
    Autorzy:
    Ćwikła-Bundyra, W.
    Powiązania:
    https://bibliotekanauki.pl/articles/778593.pdf
    Data publikacji:
    2007
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    redukcja katalityczna
    usuwanie tlenków azotu
    katalizatory metaliczne
    catalytic reduction of NO by methane
    platinum group metals catalysts
    Opis:
    Nitrogen oxide conversion to nitrogen over Pt/Al2O3, Pd/Al2O3, Rh/Al2O3 catalysts was investigated. The results of the catalytic activity investigations, with the iso-x method, showed that NO reduction by methane occurs at a reasonable rate at the temperature range 200-500°C. Alumina-supported Pd, Pt and Rh catalysts have been compared for the selective reduction of NO to N2. All the catalysts showed good activity in NO reduction by methane, giving around 80 - 90% N2 production. At moderate temperatures Pt is the most active catalyst for the removal of NO.
    Źródło:
    Polish Journal of Chemical Technology; 2007, 9, 4; 56-58
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Activity of monolithic Pd/Al2O3 catalysts in the combustion of mine ventilation air methane
    Autorzy:
    Kucharczyk, B.
    Powiązania:
    https://bibliotekanauki.pl/articles/779819.pdf
    Data publikacji:
    2011
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    katalityczne utlenianie metanu
    katalizatory monolityczne
    powietrze wentylacyjne kopalni
    catalytic oxidation of methane
    monolithic catalysts
    mine ventilation air
    Opis:
    The activity of Pd/Al2O3 catalysts increases when Pd content is increased from 1% to 2%. Among these catalysts, 2%Pd/Al2O3 shows the highest methane combustion activity. In a reduced form, the catalyst displays a higher activity than in the oxidized form. 24-hour ageing at 600oC to 800oC lowers the catalytic activity of 2%Pd/Al2O3 due to Pd crystallite sintering. After 110-hour oxidation of 1% methane in air over 2%Pd/Al2O3, conversion decreases from 100% to 88%. Upon reduction with hydrogen (performed after 24-hour ageing at 700oC and 110-hour methane oxidation), the 2%Pd/Al2O3 catalyst regains its initial activity. The high activity of Pd catalysts renders them suitable for methane removal from coal mine ventilation air at high gas fl ow velocities and temperatures lower than 600oC.
    Źródło:
    Polish Journal of Chemical Technology; 2011, 13, 4; 57-62
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Methane production during laboratory-scale co-digestion of cattle slurry with 10 wt. % of various biowastes
    Autorzy:
    Rusín, J.
    Chamrádová, K.
    Obroučka, K.
    Kuča, R.
    Powiązania:
    https://bibliotekanauki.pl/articles/778299.pdf
    Data publikacji:
    2012
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    swoista produkcja metanu
    bioodpady
    gnojowica bydlęca
    trawienie beztlenowe
    biowaste
    cattle slurry
    anaerobic co-digestion
    specific methane production
    Opis:
    The paper summarizes the results from twenty model tests of continuous one-stage mesophilic anaerobic co-digestion of cattle slurry (90 wt. %) and various biowastes (10 wt. %). Digestion was conducted in 0.06 m3 reactors with hydraulic retention times ranging from 60 to 98 days during the research period 2007-2010. Methane production intensity and specific methane production are discussed. The highest methane production intensity (0.85 mN3.m-3.d-1) was from a mixture of 63 wt. % of total solids from biscuit meal EKPO - EB and from 37 wt. % of total solids from cattle slurry. The highest specific methane production from 1 kg of added organic compounds (0.67 mN3.kgVSp-1) was given by a mixture containing 61 wt. % of total solids using spring barley Aksamit (milled grain) and 39 wt. % of total solids from cattle slurry. The highest substrate-specific methane production (0.92 mN3.kgVSp-1) was from milled grains of winter rye Aventino.
    Źródło:
    Polish Journal of Chemical Technology; 2012, 14, 1; 14-20
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
    Tytuł:
    Numerical analysis of a serial connection of two staged SOFC stacks in a CHP system fed by methane using Aspen TECH
    Autorzy:
    Pianko-Oprych, Paulina
    Palus, Mateusz
    Powiązania:
    https://bibliotekanauki.pl/articles/779502.pdf
    Data publikacji:
    2019
    Wydawca:
    Zachodniopomorski Uniwersytet Technologiczny w Szczecinie. Wydawnictwo Uczelniane ZUT w Szczecinie
    Tematy:
    Solid Oxide Fuel Cell stacks
    Combined Heat and Power system
    Balance of Plant
    BoP
    modelling
    methane
    Catalytic Partial Oxidation
    CPOx
    reformer
    steam reformer
    part and full load
    steady state
    dynamic model
    Opis:
    The objective of the study was to develop a steady-state system model in Aspen TECH using user-defined subroutines to predict the SOFC electrochemical performance. In order to achieve high overall fuel utilization and thus high electrical efficiency, a concept of Combined Heat and Power system with two-stage SOFC stacks of different number of cells was analyzed. The concept of two-stage SOFC stacks based system was developed in the framework of the FP7 EU-funded project STAGE-SOFC. The model was validated against data gathered during the operation of the proof-of-concept showing good agreement with the comparative simulation data. Following model validation, further simulations were performed for different values of fuel utilization to analyze its influence on system electrical performance. Simulation results showed that the concept of two-stage SOFC stacks configuration was viable and reliable. The model can be useful for development the optimal control strategy for system under safe conditions.
    Źródło:
    Polish Journal of Chemical Technology; 2019, 21, 1; 33-43
    1509-8117
    1899-4741
    Pojawia się w:
    Polish Journal of Chemical Technology
    Dostawca treści:
    Biblioteka Nauki
    Artykuł
      Wyświetlanie 1-14 z 14

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