Ocena wielkości emisji węglowodorów do atmosfery podczas przeładunku i magazynowania oleju napędowego w zbiornikach z dachem stałym Assessment of the amount of hydrocarbon emissions to the atmosphere during handling and storage of diesel fuel in fixed roof tanks
Diesel fuels currently constitute around 60–70% of the turnover of fuel bases in Poland. Diesel fuels are stored in vertical steel tanks with fixed roofs, which, according to applicable legal acts, do not require airtight sealing. This results in the emission of gases containing hydrocarbons to the atmosphere, which at high turnover of fuel bases generates the need to determine the concentration of hydrocarbons emitted to the atmosphere and to perform calculations of concentrations occurring at the boundary of the fuel base site. The article collects available literature data and presents the results of research on the emissions of hydrocarbons to the atmosphere that occur during handling and storage of diesel fuel in storage tanks, including the determination of the saturated vapor pressure of the hydrocarbon components of the tested diesel fuel depending on the temperature. The emissions tests were carried out by taking gas samples emitted during operations on diesel storage tanks. Analyzes of the gas samples supplied in gas-tight syringes were performed with SRI 8610C gas chromatograph equipped with a flame ionization detector (FID) and an alumina packed column. Diesel oil sample analysis was performed by gas chromatography using Shimadzu GC-2010 Plus chromatograph equipped with flame ionization detector (FID). ZB-5HT column (30 m × 0.25 mm × 0.25 µm) was used for the separation of the substances. Research has shown the amount of hydrocarbon emissions to the atmosphere depending on the type of loading operations, the degree of storage tank filling and oil temperature. The dependence of the concentration of hydrocarbons emitted from the storage tank depending on the degree of filling of the tank has been determined in the research. Results of calculations of diesel vapor pressure show convergence with most available literature data and measurement results. General design guidelines have been defined to determine the data necessary to calculate the level of hydrocarbon concentrations in atmospheric air. The research was aimed at creating the basis for the required environmental calculations, relevant in the absence of relevant literature data, necessary for the reliable determination of the amount of hydrocarbon emissions.
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